Prospect of Sulfurized Pyrolyzed Poly(acrylonitrile) (S@pPAN) Cathode Materials for Rechargeable Lithium Batteries

Yang Huijun; Chen Jiahang; Yang Jun; Wang Jiulin

摘要

Abstract >Lithium–sulfur (Li–S) batteries are one of the most promising next‐generation batteries owing to their ultra‐high theoretical energy density and that sulfur is an abundant resource. During the past 20?years, various sulfur materials have been reported. As a molecular‐scale sulfur‐composite cathode, sulfurized pyrolyzed poly(acrylonitrile) (S@pPAN) exhibits several competitive advantages in terms of its electrochemical behavior. Although it was first reported in 2002 S@pPAN is currently attracting increasing attention. In this Minireview, we summarize its molecular model and explore the correlation between its structure and its exceptional electrochemical performance. We classify the modification strategies into three types, including material improvement, binder, and electrolyte screening. Several research and development directions are also suggested. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >锂 - 硫（LI-S）电池是由于其超高理论能量密度的最有前一代电池之一，并且硫是一种丰富的资源。在过去的20年中，已经报道了各种硫材料。作为分子级硫 - 复合阴极，硫化热解的聚（丙烯腈）（丙烯腈）（丙烯腈）就其电化学行为而言表现出几种竞争优势。虽然它是2002年首次报道的@PPP目前吸引了不断的关注。在这个Miniview中，我们总结了其分子模型，并探讨了其结构与其特殊电化学性能之间的相关性。我们将修改策略分为三种类型，包括材料改进，粘合剂和电解质筛选。还提出了几项研究和发展方向。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第19期</span><b style="margin: 0 2px;">|</b><span>共13页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Huijun&option=202" target="_blank" rel="nofollow">Yang Huijun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Jiahang&option=202" target="_blank" rel="nofollow">Chen Jiahang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Jun&option=202" target="_blank" rel="nofollow">Yang Jun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Jiulin&option=202" target="_blank" rel="nofollow">Wang Jiulin;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Shanghai Electrochemical Energy Devices Research CenterShanghai Jiao Tong UniversityShanghai 200240 China;</p> <p>Shanghai Electrochemical Energy Devices Research CenterShanghai Jiao Tong UniversityShanghai 200240 China;</p> <p>Shanghai Electrochemical Energy Devices Research CenterShanghai Jiao Tong UniversityShanghai 200240 China;</p> <p>Shanghai Electrochemical Energy Devices Research CenterShanghai Jiao Tong UniversityShanghai 200240 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=battery safety&option=203" rel="nofollow">battery safety;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=interfacial regulation&option=203" rel="nofollow">interfacial regulation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium–sulfur batteries&option=203" rel="nofollow">lithium–sulfur batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=S@pPAN cathode&option=203" rel="nofollow">S@pPAN cathode;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=solid–solid conversion&option=203" rel="nofollow">solid–solid conversion;</a> </p> <div class="translation"> 机译：电池安全;界面调节;锂 - 硫电池;S @ PPAN阴极;固体 - 固体转换; 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