Dimensional Reduction of Cs2AgBiBr6 : A 2D Hybrid Double Perovskite with Strong Polarization Sensitivity

Li Yaobin; Yang Tao; Xu Zhiyun; Liu Xitao; Huang Xiaoying; Han Shiguo; Liu Yi; Li Maofan; Luo Junhua; Sun Zhihua

摘要

Abstract > By dimensional reduction of the 3D motif of Cs <sub>2</sub> AgBiBr <sub>6</sub> , a lead‐free 2D hybrid double perovskite, ( i ‐PA) <sub>2</sub> CsAgBiBr <sub>7</sub> ( 1, i ‐PA=isopentylammonium), was successfully designed. It adopts a quantum‐confined bilayered structure with alternating organic and inorganic sheets. Strikingly, the unique 2D architecture endows it highly anisotropic nature of physical properties, including electric conductivity and optical absorption (the ratio α <sub>b</sub> / α <sub>c</sub> =1.9 at 405?nm). Such anisotropy attributes result in the strong polarization‐sensitive responses with large dichroic ratios up to 1.35, being comparable to some 2D inorganic materials. This is the first study on the hybrid double perovskites with strong polarization sensitivity. A crystal device of 1 also exhibits rapid response speed (ca. 200?μs) and excellent stabilities. The family of 2D hybrid double perovskites are promising optoelectronic candidates, and this work paves a new pathway for exploring new green polarization‐sensitive materials. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 通过CS的3D图案的维度减少 <sub> 2 </ sub> AGBIBR. <sub> 6 </ sub> ，无铅2D杂交双钙钛矿，（我</ i> -PA） <sub> 2 </ sub> csagbibri <sub> 7 </ sub> （ 1，</ b> 我</ i> -Pa =等戊基铵），成功设计。它采用具有交替的有机和无机片的量子狭窄的双层结构。令人惊讶的是，独特的2D架构赋予物理性质的极大各向异性性质，包括导电性和光学吸收（比率 α</ i> <sub> b </ sub> / α</ i> <sub> c </ sub> = 1.9在405？nm处）。这种各向异性属性导致具有高达1.35的大二向色比的强偏振敏感反应，与一些2D无机材料相当。这是具有强极化敏感性强的杂种双钙锌矿的第一研究。一个晶体装置 1 </ b> 还表现出快速的响应速度（约200？μs）和优异的稳定性。 2D Hybrid Double Perovskites的家庭是有前途的光电候选者，这项工作铺设了一种新的途径，用于探索新的绿色偏振敏感材料。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第9期</span><b style="margin: 0 2px;">|</b><span>共5页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yaobin&option=202" target="_blank" rel="nofollow">Li Yaobin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Tao&option=202" target="_blank" rel="nofollow">Yang Tao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Zhiyun&option=202" target="_blank" rel="nofollow">Xu Zhiyun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Xitao&option=202" target="_blank" rel="nofollow">Liu Xitao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Xiaoying&option=202" target="_blank" rel="nofollow">Huang Xiaoying;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Han Shiguo&option=202" target="_blank" rel="nofollow">Han Shiguo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Yi&option=202" target="_blank" rel="nofollow">Liu Yi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Maofan&option=202" target="_blank" rel="nofollow">Li Maofan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Luo Junhua&option=202" target="_blank" rel="nofollow">Luo Junhua;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Zhihua&option=202" target="_blank" rel="nofollow">Sun Zhihua;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> <p>State Key Laboratory of Structural ChemistryChinese Academy of SciencesFuzhou Fujian 350002 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dimensional reduction&option=203" rel="nofollow">dimensional reduction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hybrid double perovskites&option=203" rel="nofollow">hybrid double perovskites;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lead-free perovskites&option=203" rel="nofollow">lead-free perovskites;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polarization sensitivity&option=203" rel="nofollow">polarization sensitivity;</a> </p> <div class="translation"> 机译：尺寸减少;杂交双钙质;无铅蠕动;极化敏感性; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028162697.html">Dimensional Reduction of Cs2AgBiBr6 : A 2D Hybrid 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class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020311389175.html">接地网腐蚀速率弱极化检测及强极化状态评价方法研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=黄小琼&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 黄小琼</a> <span> . 2015</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120113753271.html">一种具有优异非线性光学性能Cs2AgBiBr6双钙钛矿薄膜的制备方法</a> <b>[P]</b> . <span> 中国专利： CN113753951A </span> <span> . 2021-12-07</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120108871959.html">具有强分蘖能力的多穗型超级杂交稻两用核不育系选育方法</a> <b>[P]</b> . <span> 中国专利： CN106386473A </span> <span> . 2017-02-15</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130409862746.html">HALIDE DOUBLE PEROVSKITE Cs2AgBiBr6 SOLAR-CELL ABSORBER HAVING LONG CARRIER LIFETIMES</a> <b>[P]</b> . <span> 外国专利：  US2017194101A1 </span> <span> . 2017-07-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：卤化物双钙钛矿Cs2AgBiBr6太阳能吸收器寿命长 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130408749072.html">2D/3D POLARIZATION SWITCHING TOUCH SCREEN PANEL SWITCHABLE LENS TOUCH SCREEN PANEL AND 2-DIMENSIONAL AND 3-DIMENSIONAL IMAGE DISPLAY DEVICE HAVING THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR20170019006A </span> <span> . 2017-02-21</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有相同功能的2D / 3D偏光切换触摸屏面板可切换镜头触摸屏面板和2维和3维图像显示设备 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130408613713.html">2D/3D POLARIZATION SWITCHING TOUCH SCREEN PANEL SWITCHABLE LENS TOUCH SCREEN PANEL AND 2-DIMENSIONAL AND 3-DIMENSIONAL IMAGE DISPLAY DEVICE HAVING THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR101721325B1 </span> <span> . 2017-03-30</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有相同功能的2D / 3D偏光切换触摸屏面板可切换镜头触摸屏面板和2维和3维图像显示设备 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704028162697','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> 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