The Structure of Water Bonded to Phosphate Groups at the Electrified Zwitterionic Phospholipid Membranes/Aqueous Interface

Li Shanshan; Wu Lie; Zhang Xiaofei; Jiang Xiue

摘要

Abstract > Gaining insight into the water structure at the electrified phospholipid membranes/aqueous interface is vital and essential for elucidating the mechanism of many biochemical reactions, but still remains a formidable challenge. Herein, based on the superiority of surface enhanced infrared absorption (SEIRA) spectroscopy combined with electrochemistry in interfacial analysis, the evolution of local water structure at the zwitterionic phospholipid membranes/aqueous interface with an external electric field is revealed by means of ion perturbation. The strongly hydrogen‐bonded water directly bonded to the phosphate groups (PO <sub>2</sub> ? ) has a strong mechanical strength to resist potential perturbations, and that portion of water greatly affects the electrostatic properties of the phospholipid membranes. This study innovates the basic understanding of electric double layer (EDL) at the membranes/aqueous interface. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在阐明电气化的磷脂膜/水界面处的水结构的洞察力至关重要，阐明许多生化反应的机制，但仍然是一个强大的挑战。这里，基于表面增强的红外吸收（Seira）光谱与电化学在界面分析中结合的优势，通过离子扰动揭示了杂散磷脂膜/水性界面中局部水结构的演变。通过离子扰动揭示了外部电场。强氢键合水直接粘合到磷酸盐基团（PO <sub> 2 </ sub> ？</ sup> ）具有强大的机械强度来抵抗潜在的扰动，并且该部分的水极大地影响了磷脂膜的静电性质。本研究创新了对膜/水界面的电双层（EDL）的基本理解。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共4页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Shanshan&option=202" target="_blank" rel="nofollow">Li Shanshan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Lie&option=202" target="_blank" rel="nofollow">Wu Lie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xiaofei&option=202" target="_blank" rel="nofollow">Zhang Xiaofei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Xiue&option=202" target="_blank" rel="nofollow">Jiang Xiue;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Electroanalytical ChemistryChinese Academy of SciencesChangchun 130022 Jilin China;</p> <p>State Key Laboratory of Electroanalytical ChemistryChinese Academy of SciencesChangchun 130022 Jilin China;</p> <p>State Key Laboratory of Electroanalytical ChemistryChinese Academy of SciencesChangchun 130022 Jilin China;</p> <p>State Key Laboratory of Electroanalytical ChemistryChinese Academy of SciencesChangchun 130022 Jilin China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dipole potential&option=203" rel="nofollow">dipole potential;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=interfacial electric field&option=203" rel="nofollow">interfacial electric field;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=interfacial water&option=203" rel="nofollow">interfacial water;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ions perturbation&option=203" rel="nofollow">ions perturbation;</a> </p> <div class="translation"> 机译：偶极电位;界面电场;界面水;离子扰动; 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href="/academic-conference-cn_meeting-17466_thesis/020221836649.html">离子在β型分子筛膜修饰水/1,2-二氯乙烷界面上的转移反应</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . </a> <span> <a href="/conference-cn-17466/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第十届全国电分析化学学术会议 </a> <span> <span> . 2008</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020315323715.html">含亲水辅助基团离子交换膜的制备及其扩散渗析性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=纪文根&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 纪文根</a> <span> . 2020</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120104109544.html">一种不含吸电子基团的醚氧基对位季铵结构阴离子交换膜及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN111430763A </span> <span> . 2020-07-17</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120214918599.html">水性负离子净醛肌理壁膜浆复合结构</a> <b>[P]</b> . <span> 中国专利： CN215368369U </span> <span> . 2021-12-31</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130433160268.html">Aqueous systems containing phospholipid, surfactant and phosphate ester for water-insoluble materials</a> <b>[P]</b> . <span> 外国专利：  US2008096782A1 </span> <span> . 2008-04-24</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于非水溶性材料的含有磷脂，表面活性剂和磷酸酯的水性体系 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130417743288.html">"The structures of membrane, method of treating a multipicidade of porous substrates that apresnetam condutes tubular formed inside them to condition the substrates for the formation of the membrane method to treat a variety of porous substrates which have consuites tubular formed den Four of them to form membranes in these conduits.Module, method for forming zeolite membranes on the internal surfaces of a multiplicity of conduits, usually in the monolith to another method for removal of water from an organic liquid through the conduits in a memebranas structures.Methods the puricu00c3u00c7u00c3o water containing salt or other contaminants which include continues the water through conduits into one or more membrane structures.</a> <b>[P]</b> . <span> 外国专利：  BRPI0808229A2 </span> <span> . 2014-07-08</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：膜的结构，处理多孔基质的多种方法的方法，即presnetam渗出在其内部形成的管状物以调节基质的形成膜的方法，以处理各种具有管状相结合的多孔基质的膜。在多个导管的内表面形成沸石膜的方法，通常是整体式;另一种方法是通过膜结构中的导管从有机液体中除去水。含有盐或其他污染物的水，其中包括通过导管将水连续引入一个或多个膜结构的水。 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130443716780.html">Phospholipid composition useful for preparing cosmetic compositions comprises a phospholipid membrane former, a phenoxylalkanol solvent and water</a> <b>[P]</b> . <span> 外国专利：  DE10128315A1 </span> <span> . 2003-01-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于制备化妆品组合物的磷脂组合物包含磷脂膜形成剂，苯氧基链烷醇溶剂和水 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" 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