Structure‐Independent Conductance of Thiophene‐Based Single‐Stacking Junctions

Li Xiaohui; Wu Qingqing; Bai Jie; Hou Songjun; Jiang Wenlin; Tang Chun; Song Hang; Huang Xiaojuan; Zheng Jueting; Yang Yang; Liu Junyang; Hu Yong; Shi Jia; Liu Zitong; Lambert Colin J.; Zhang Deqing; Hong Wenjing

摘要

Abstract >The experimental investigation of intermolecular charge transport in π‐conjugated materials is challenging. Herein, we describe the investigation of charge transport through intermolecular and intramolecular paths in single‐molecule and single‐stacking thiophene junctions by the mechanically controllable break junction (MCBJ) technique. We found that the ability for intermolecular charge transport through different single‐stacking junctions was approximately independent of the molecular structure, which contrasts with the strong length dependence of conductance in single‐molecule junctions with the same building blocks, and the dominant charge‐transport path of molecules with two anchors transited from an intramolecular to an intermolecular path when the degree of conjugation increased. An increase in conjugation further led to higher binding probability owing to the variation in binding energies, as supported by DFT calculations. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >π-共轭材料中分子间电荷输送的实验研究是具有挑战性的。在此，通过机械可控的断裂结（MCBJ）技术描述通过单分子中的分子和分子内径和单分子分子内途径的电荷输送研究。我们发现，通过不同的单堆叠结的分子间电荷传输的能力大致与分子结构相比，与具有相同构建块的单分子交叉点的电导率强度依赖性相比，以及主力电荷传输路径对比。当缀合程度增加时，分子与分子内转变为分子内的分子间路径。由于DFT计算的支持，缀合的增加进一步导致了更高的结合概率。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第8期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Xiaohui&option=202" target="_blank" rel="nofollow">Li Xiaohui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Qingqing&option=202" target="_blank" rel="nofollow">Wu Qingqing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bai Jie&option=202" target="_blank" rel="nofollow">Bai Jie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hou Songjun&option=202" target="_blank" rel="nofollow">Hou Songjun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Wenlin&option=202" target="_blank" rel="nofollow">Jiang Wenlin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tang Chun&option=202" target="_blank" rel="nofollow">Tang Chun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Song Hang&option=202" target="_blank" rel="nofollow">Song Hang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Xiaojuan&option=202" target="_blank" rel="nofollow">Huang Xiaojuan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zheng Jueting&option=202" target="_blank" rel="nofollow">Zheng Jueting;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Yang&option=202" target="_blank" rel="nofollow">Yang Yang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Junyang&option=202" target="_blank" rel="nofollow">Liu Junyang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hu Yong&option=202" target="_blank" rel="nofollow">Hu Yong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shi Jia&option=202" target="_blank" rel="nofollow">Shi Jia;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Zitong&option=202" target="_blank" rel="nofollow">Liu Zitong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lambert Colin J.&option=202" target="_blank" rel="nofollow">Lambert Colin J.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Deqing&option=202" target="_blank" rel="nofollow">Zhang Deqing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hong Wenjing&option=202" target="_blank" rel="nofollow">Hong Wenjing;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>Department of PhysicsLancaster UniversityLancaster LA1 4YB UK;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>Department of PhysicsLancaster UniversityLancaster LA1 4YB UK;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesZhongguancun North First Street 2 Beijing China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesZhongguancun North First Street 2 Beijing China;</p> <p>Department of PhysicsLancaster UniversityLancaster LA1 4YB UK;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesZhongguancun North First Street 2 Beijing China;</p> <p>State Key Laboratory of Physical Chemistry of Solid Surfaces iChEMXiamen UniversitySiming South Road Xiamen China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=conducting materials&option=203" rel="nofollow">conducting materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=conjugation&option=203" rel="nofollow">conjugation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=mechanically controllable break junctions&option=203" rel="nofollow">mechanically controllable break junctions;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=intermolecular charge transport&option=203" rel="nofollow">intermolecular charge transport;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thiophene junctions&option=203" rel="nofollow">thiophene junctions;</a> </p> <div class="translation"> 机译：导电材料;共轭;机械控制的断裂连接;分子间电荷运输;噻吩连接; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028162016.html">Structure‐Independent Conductance of Thiophene‐Based Single‐Stacking Junctions</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Xiaohui&option=202" target="_blank" rel="nofollow" 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