Strong, Self‐Healable, and Recyclable Visible‐Light‐Responsive Hydrogel Actuators

Jiang Zhen; Tan Ming Li; Taheri Mahdiar; Yan Qiao; Tsuzuki Takuya; Gardiner Michael G.; Diggle Broden; Connal Luke A.

摘要

Abstract >The most pressing challenges for light‐driven hydrogel actuators include reliance on UV light, slow response, poor mechanical properties, and limited functionalities. Now, a supramolecular design strategy is used to address these issues. Key is the use of a benzylimine‐functionalized anthracene group, which red‐shifts the absorption into the visible region and also stabilizes the supramolecular network through π–π interactions. Acid–ether hydrogen bonds are incorporated for energy dissipation under mechanical deformation and maintaining hydrophilicity of the network. This double‐crosslinked supramolecular hydrogel developed via a simple synthesis exhibits a unique combination of high strength, rapid self‐healing, and fast visible‐light‐driven shape morphing both in the wet and dry state. As all of the interactions are dynamic, the design enables the structures to be recycled and reprogrammed into different 3D objects. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >光驱动水凝胶执行器的最紧迫挑战包括依赖于UV光，慢响应，机械性能差和有限的功能。现在，使用超分子设计策略来解决这些问题。键是使用苄胺官能化的蒽基，其向可见区域的吸收使吸收率并通过π-π相互作用稳定超分子网络。酸 - 醚氢键掺入，用于在机械变形下的能量耗散并保持网络的亲水性。通过简单合成开发的这种双交联的超分子水凝胶具有高强度，快速的自愈和在湿和干燥状态下的高强度，快速自愈和快速可见光的形状变形的独特组合。随着所有交互都是动态的，设计使结构能够被回收并重新编程为不同的3D对象。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第18期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Zhen&option=202" target="_blank" rel="nofollow">Jiang Zhen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tan Ming Li&option=202" target="_blank" rel="nofollow">Tan Ming Li;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Taheri Mahdiar&option=202" target="_blank" rel="nofollow">Taheri Mahdiar;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Qiao&option=202" target="_blank" rel="nofollow">Yan Qiao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tsuzuki Takuya&option=202" target="_blank" rel="nofollow">Tsuzuki Takuya;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gardiner Michael G.&option=202" target="_blank" rel="nofollow">Gardiner Michael G.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Diggle Broden&option=202" target="_blank" rel="nofollow">Diggle Broden;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Connal Luke A.&option=202" target="_blank" rel="nofollow">Connal Luke A.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Research School of ChemistryAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of ChemistryAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of Electrical Energy and Materials EngineeringAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of ChemistryAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of Electrical Energy and Materials EngineeringAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of ChemistryAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of ChemistryAustralian National UniversityCanberra ACT 2601 Australia;</p> <p>Research School of ChemistryAustralian National UniversityCanberra ACT 2601 Australia;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=actuators&option=203" rel="nofollow">actuators;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=anthracene&option=203" rel="nofollow">anthracene;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photoresponsive hydrogels&option=203" rel="nofollow">photoresponsive hydrogels;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=self-healing&option=203" rel="nofollow">self-healing;</a> </p> <div class="translation"> 机译：执行器;蒽;光响应水凝胶;自我修复; 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