Chemo‐ and Magnetotaxis of Self‐Propelled Light‐Emitting Chemo‐electronic Swimmers

Salinas Gerardo; Dauphin Alice L.; Colin Camille; Villani Elena; Arbault Stéphane; Bouffier Laurent; Kuhn Alexander

摘要

Abstract > Miniaturized autonomous chemo‐electronic swimmers, based on the coupling of spontaneous oxidation and reduction reactions at the two poles of light‐emitting diodes (LEDs), are presented as chemotactic and magnetotactic devices. In homogeneous aqueous media, random motion caused by a bubble‐induced propulsion mechanism is observed. However, in an inhomogeneous environment, the self‐propelled devices exhibit positive chemotactic behavior, propelling themselves along a pH or ionic strength gradient (?pH and ? I , respectively) in order to reach a thermodynamically higher active state. In addition, the intrinsic permanent magnetic moment of the LED allows self‐orientation in the terrestrial magnetic field or following other external magnetic perturbations, which enables a directional motion control coupled with light emission. The interplay between chemotaxis and magnetotaxis allows fine‐tuning of the dynamic behavior of these swimmers. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 基于发光二极管（LED）的两极的自发氧化和还原反应的耦合为趋化性和磁通时路，小型化自主化疗。在均相水性介质中，观察由气泡诱导的推进机构引起的随机运动。然而，在不均匀的环境中，自推进装置表现出阳性趋化性，沿pH或离子强度梯度引出（αpH和？我</ i> 分别）以达到热力学上更高的活性状态。另外，LED的内在永磁磁矩允许在地面磁场中的自定向或跟随其他外部磁扰动，这使得能够与发光耦合的定向运动控制。趋化性和Magnetotaxis之间的相互作用允许微调这些游泳运动员的动态行为。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第19期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Salinas Gerardo&option=202" target="_blank" rel="nofollow">Salinas Gerardo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dauphin Alice L.&option=202" target="_blank" rel="nofollow">Dauphin Alice L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Colin Camille&option=202" target="_blank" rel="nofollow">Colin Camille;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Villani Elena&option=202" target="_blank" rel="nofollow">Villani Elena;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Arbault Stéphane&option=202" target="_blank" rel="nofollow">Arbault Stéphane;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bouffier Laurent&option=202" target="_blank" rel="nofollow">Bouffier Laurent;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kuhn Alexander&option=202" target="_blank" rel="nofollow">Kuhn Alexander;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> <p>CNRS UMR 5255Univ. Bordeaux33607 Pessac France;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=chemotaxis&option=203" rel="nofollow">chemotaxis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electronic swimmers&option=203" rel="nofollow">electronic swimmers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=light emission&option=203" rel="nofollow">light emission;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=magnetotaxis&option=203" rel="nofollow">magnetotaxis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=pH gradients&option=203" rel="nofollow">pH gradients;</a> </p> <div class="translation"> 机译：趋化性;电子游泳者;发光;MarageCaxis;pH梯度; 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