Selective Expression of Chromophores in a Single Molecule: Soft Organic Crystals Exhibiting Full‐Colour Tunability and Dynamic Triplet‐Exciton Behaviours

Li Wenlang; Huang Qiuyi; Mao Zhu; Zhao Juan; Wu Huiyan; Chen Junru; Yang Zhan; Li Yang; Yang Zhiyong; Zhang Yi; Aldred Matthew P.; Chi Zhenguo

摘要

Abstract >Soft luminescent materials are attractive for optoelectronic applications, however, switching dominant chromophores for property enrichment remains a challenge. Herein, we report the first case of a soft organic molecule (DOS) featuring selective expression of chromophores. In response to various external stimuli, different chromophores of DOS can take turns working through conformation changes, exhibiting full‐colour emissions peaking from 469?nm to 583?nm from ten individual single crystals. Dynamic triplet‐exciton behaviours including thermally activated delayed fluorescence (TADF), room‐temperature phosphorescence (RTP), mechanoluminescence (ML), and distinct mechano‐responsive luminescence (MRL) can all be realized. This novel designed DOS molecule provides a multifunctional platform for detection of volatile organic compounds (VOCs), multicolour dynamic displays, sensing, anticounterfeiting, and hopefully many others. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P>软发光材料对于光电应用具有吸引力，但是，用于物质富集的转换显性发色团仍然是一个挑战。在此，我们报告了具有发色团的选择性表达的软有机分子（DOS）的第一种情况。响应于各种外部刺激，不同的DOS发色团可以通过构象变化，表现出从10个单个单个晶体的469℃至583℃达到峰值的全色排放量。可以实现动态三重态 - 激子行为，包括热活化的延迟荧光（TADF），室温磷光（RTP），机械发光（ML）和不同的机械响应发光（MRL）。该新型设计的DOS分子为检测挥发性有机化合物（VOC），多色动态显示器，感应，射行，希望许多其他多功能平台提供多功能平台。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第9期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Wenlang&option=202" target="_blank" rel="nofollow">Li Wenlang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Qiuyi&option=202" target="_blank" rel="nofollow">Huang Qiuyi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mao Zhu&option=202" target="_blank" rel="nofollow">Mao Zhu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Juan&option=202" target="_blank" rel="nofollow">Zhao Juan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Huiyan&option=202" target="_blank" rel="nofollow">Wu Huiyan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Junru&option=202" target="_blank" rel="nofollow">Chen Junru;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Zhan&option=202" target="_blank" rel="nofollow">Yang Zhan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yang&option=202" target="_blank" rel="nofollow">Li Yang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Zhiyong&option=202" target="_blank" rel="nofollow">Yang Zhiyong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Yi&option=202" target="_blank" rel="nofollow">Zhang Yi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Aldred Matthew P.&option=202" target="_blank" rel="nofollow">Aldred Matthew P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chi Zhenguo&option=202" target="_blank" rel="nofollow">Chi Zhenguo;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>Instrumental Analysis and Research Center (IARC)Sun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> <p>PCFM LabSun Yat-sen UniversityGuangzhou 510275 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=crystal engineering&option=203" rel="nofollow">crystal engineering;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=full-colour emission&option=203" rel="nofollow">full-colour emission;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=luminescence&option=203" rel="nofollow">luminescence;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=soft molecule&option=203" rel="nofollow">soft molecule;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=triplet-exciton&option=203" rel="nofollow">triplet-exciton;</a> </p> <div class="translation"> 机译：水晶工程;全彩发射;发光;软分子;三重素 - 激子; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028161760.html">Selective Expression of Chromophores in a Single Molecule: Soft Organic Crystals Exhibiting Full‐Colour Tunability and Dynamic Triplet‐Exciton 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