Intrinsic Facet‐Dependent Reactivity of Well‐Defined BiOBr Nanosheets on Photocatalytic Water Splitting

Shi Ming; Li Guanna; Li Jianming; Jin Xu; Tao Xiaoping; Zeng Bin; Pidko Evgeny A.; Li Rengui; Li Can

摘要

Abstract >Surface atomic arrangement and coordination of photocatalysts highly exposed to different crystal facets significantly affect the photoreactivity. However, controversies on the true photoreactivity of a specific facet in heterogeneous photocatalysis still exits. Herein, we exemplified well‐defined BiOBr nanosheets dominating with respective facets, (001) and (010), to track the reactivity of crystal facets for photocatalytic water splitting. The real photoreactivity of BiOBr‐(001) were evidenced to be significantly higher than BiOBr‐(010) for both hydrogen production and oxygen evolution reactions. Further in?situ photochemical probing studies verified the distinct reactivity is not only owing to the highly exposed facets, but dominated by the co‐exposing facets, leading to an efficient spatial separation of photogenerated charges and further making the oxidation and reduction reactions separately occur with different reaction rates, which ordains the fate of the true photoreactivity. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >表面原子布置和光催化剂的光催化剂高度暴露于不同的晶面显着影响光反应性。然而，异构光催化在异构光催化中的特定方面的真实光反应性的争议仍然出现。在此，我们示出了定义明确的BIOBR纳米片，其与各个刻面，（001）和（010）进行主导，以跟踪光催化水分裂的晶面的反应性。 BioBR-（001）的真实光反应性被证明是显着高于BioBR-（010），用于氢气产生和氧气进化反应。进一步进一步？原位光化学探测研究验证了不同的反应性不仅由于高度暴露的刻面，而是由共同暴露的小平面所导样，导致光生电电荷的有效空间分离，并进一步使氧化和还原反应分别发生不同的反应速率，该反应速率被定为真正的光反应性的命运。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shi Ming&option=202" target="_blank" rel="nofollow">Shi Ming;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Guanna&option=202" target="_blank" rel="nofollow">Li Guanna;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Jianming&option=202" target="_blank" rel="nofollow">Li Jianming;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jin Xu&option=202" target="_blank" rel="nofollow">Jin Xu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tao Xiaoping&option=202" target="_blank" rel="nofollow">Tao Xiaoping;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zeng Bin&option=202" target="_blank" rel="nofollow">Zeng Bin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pidko Evgeny A.&option=202" target="_blank" rel="nofollow">Pidko Evgeny A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Rengui&option=202" target="_blank" rel="nofollow">Li Rengui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Can&option=202" target="_blank" rel="nofollow">Li Can;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of CatalysisThe Collaborative Innovation Center of Chemistry for Energy Materials (iChem-2011)Dalian 116023 China;</p> <p>Inorganic Systems EngineeringDelft University of TechnologyVan der Maasweg 9 2629 HZ Delft Netherlands;</p> <p>Research Institute of Petroleum Exploration &</p> <p>Development (RIPED)PetroChinaBeijing 100083 China;</p> <p>Research Institute of Petroleum Exploration &</p> <p>Development (RIPED)PetroChinaBeijing 100083 China;</p> <p>State Key Laboratory of CatalysisThe Collaborative Innovation Center of Chemistry for Energy Materials (iChem-2011)Dalian 116023 China;</p> <p>State Key Laboratory of CatalysisThe Collaborative Innovation Center of Chemistry for Energy Materials (iChem-2011)Dalian 116023 China;</p> <p>Inorganic Systems EngineeringDelft University of TechnologyVan der Maasweg 9 2629 HZ Delft Netherlands;</p> <p>State Key Laboratory of CatalysisThe Collaborative Innovation Center of Chemistry for Energy Materials (iChem-2011)Dalian 116023 China;</p> <p>State Key Laboratory of CatalysisThe Collaborative Innovation Center of Chemistry for Energy Materials (iChem-2011)Dalian 116023 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=BiOBr&option=203" rel="nofollow">BiOBr;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=facet-dependency&option=203" rel="nofollow">facet-dependency;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=intrinsic reactivity&option=203" rel="nofollow">intrinsic reactivity;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photocatalysis&option=203" rel="nofollow">photocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=water splitting&option=203" rel="nofollow">water splitting;</a> </p> <div class="translation"> 机译：biobr;刻面依赖;内在反应性;光催化;水分裂; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> 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water soluble graphene nanosheets</a> <b>[P]</b> . <span> 外国专利：  KR101290690B1 </span> <span> . 2013-07-29</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：纯净水溶性石墨烯纳米片的光催化合成 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130400665145.html">WATER-SOLUBLE ORGANIC PHOTOCATALYST AND WATER SPLITTING HYDROGEN EVOLUTION PHOTOCATALYTIC SYSTEM USING THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR102062869B1 </span> <span> . 2020-01-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：水溶性有机光催化剂和水分解氢演化光催化剂体系的相同 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> 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