Amidation‐Dominated Re‐Assembly Strategy for Single‐Atom Design/Nano‐Engineering: Constructing Ni/S/C Nanotubes with Fast and Stable K‐Storage

Yi Zheng; Jiang Song; Tian Jie; Qian Yong; Chen Shimou; Wei Shiqiang; Lin Ning; Qian Yitai

摘要

Abstract > An amidation‐dominated re‐assembly strategy is developed to prepare uniform single atom Ni/S/C nanotubes. In this re‐assembly process, a single‐atom design and nano‐structured engineering are realized simultaneously. Both the NiO <sub>5</sub> single‐atom active centers and nanotube framework endow the Ni/S/C ternary composite with accelerated reaction kinetics for potassium‐ion storage. Theoretical calculations and electrochemical studies prove that the atomically dispersed Ni could enhance the convention kinetics and decrease the decomposition energy barrier of the chemically‐absorbed small‐molecule sulfur in Ni/S/C nanotubes, thus lowering the electrode reaction overpotential and resistance remarkably. The mechanically stable nanotube framework could well accommodate the volume variation during potassiation/depotassiation process. As a result, a high K‐storage capacity of 608?mAh?g ?1 at 100?mA?g ?1 and stable cycling capacity of 330.6?mAh?g ?1 at 1000?mA?g ?1 after 500 cycles are achieved. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 开发了酰胺化主导的重组策略以制备均匀的单个原子Ni / S / C纳米管。在该重新装配过程中，同时实现单原子设计和纳米结构工程。都是nio <sub> 5 </ sub> 单原子活性中心和纳米管框架赋予Ni / S / C三元复合材料，加速反应动力学进行钾离子储存。理论计算和电化学研究证明原子分散的Ni可以增强公法动力学并降低在Ni / S / C纳米管中的化学吸收的小分子硫的分解能量屏障，从而降低电极反应的超向和阻力显着。机械稳定的纳米管框架可以很好地适应钾/沉积过程中的体积变化。结果，高k储存容量为608？mah？g ？1 </ sup> 在100？ma？g ？1 </ sup> 稳定的骑行能力为330.6？MAH？G ？1 </ sup> 在1000？ma？g ？1 </ sup> 实现500次循环后。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yi Zheng&option=202" target="_blank" rel="nofollow">Yi Zheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Song&option=202" target="_blank" rel="nofollow">Jiang Song;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Jie&option=202" target="_blank" rel="nofollow">Tian Jie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qian Yong&option=202" target="_blank" rel="nofollow">Qian Yong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Shimou&option=202" target="_blank" rel="nofollow">Chen Shimou;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wei Shiqiang&option=202" target="_blank" rel="nofollow">Wei Shiqiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Ning&option=202" target="_blank" rel="nofollow">Lin Ning;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qian Yitai&option=202" target="_blank" rel="nofollow">Qian Yitai;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Applied ChemistryUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> <p>Department of Applied ChemistryUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> <p>Experimental Center of Engineering and Material ScienceUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> <p>Department of Applied ChemistryUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> <p>Beijing Key Laboratory of Ionic Liquid Clean ProcessChinese Academy of SciencesBeijing 100190 P. R. China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> <p>Department of Applied ChemistryUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> <p>Department of Applied ChemistryUniversity of Science and Technology of ChinaHefei Anhui 230026 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=kinetics&option=203" rel="nofollow">kinetics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=K-ion batteries&option=203" rel="nofollow">K-ion batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoengineering&option=203" rel="nofollow">nanoengineering;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=single-atom Ni&option=203" rel="nofollow">single-atom Ni;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=small-molecule sulfur&option=203" rel="nofollow">small-molecule sulfur;</a> </p> <div class="translation"> 机译：动力学;K离子电池;纳米工程;单颗粒;小分子硫; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028161568.html">Amidation‐Dominated Re‐Assembly Strategy for Single‐Atom Design/Nano‐Engineering: Constructing Ni/S/C Nanotubes 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href="/academic-conference-cn_meeting-29301_thesis/020222172192.html">用于稳定和单轴扫描的快速控制反射镜结构与性能</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张洪涛&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张洪涛</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=尹福昌&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,尹福昌</a> <span> <a href="/conference-cn-29301/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 中国仪器仪表学会第六次全国会员代表大会暨学术会议 </a> <span> <span> . 2003</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314738415.html">多酸辅助合成铁基多孔纳米管与钒单原子催化剂用于小分子高效活化</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=林红&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 林红</a> <span> . 2019</span> </span> </div> </li> </ul> <ul 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carbon nanotube thin film manufacturing method and manufacturing method of a carbon nanotube FET electronic devices</a> <b>[P]</b> . <span> 外国专利：  JP4899368B2 </span> <span> . 2012-03-21</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：金属单壁碳纳米管的破坏性如何，半导体单壁碳纳米管组件的制造方法，半导体单壁碳纳米管薄膜的制造方法，半导体单壁碳纳米管的破坏性方法，金属单壁碳纤维纳米管集合体的制造方法，金属单壁碳纳米管薄膜的制造方法以及碳纳米管FET电子器件的制造方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130413679821.html">ALIGNED SINGLE-WALLED CARBON NANOTUBE ASSEMBLY, BULK ALIGNED SINGLE-WALLED CARBON NANOTUBE ASSEMBLY, POWDER-LIKE ALIGNED SINGLE-WALLED CARBON NANOTUBE ASSEMBLY, AND METHOD FOR PRODUCING SAME</a> <b>[P]</b> . <span> 外国专利：  EP2383225A4 </span> <span> . 2015-12-09</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: 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