A Chiral Reduced‐Dimension Perovskite for an Efficient Flexible Circularly Polarized Light Photodetector

Wang Lin; Xue Yongxiang; Cui Minghuan; Huang Yanmin; Xu Hongyu; Qin Chaochao; Yang Jien; Dai Haitao; Yuan Mingjian

摘要

Abstract > Chiral quasi‐2D perovskite single crystals (SCs) were investigated for their circular polarized light (CPL) detecting capability. Quasi‐2D chiral perovskites, [( R )‐β‐MPA] <sub>2</sub> MAPb <sub>2</sub> I <sub>7</sub> (( R )‐β‐MPA=( R )‐(+)‐β‐methylphenethylamine, MA=methylammonium), have intrinsic chirality and the capability to distinguish different polarization states of CPL photons. Corresponding quasi‐2D SCs CPL photodetector exhibit excellent detection performance. In particular, our device responsivity is almost one order of magnitude higher than the reported 2D perovskite CPL detectors to date. The crystallization dynamics of the film were modulated to facilitate its carrier transport. Parallel oriented perovskite films with a homogeneous energy landscape is crucial to maximize the carrier collection efficiency. The photodetector also exhibits superior mechanical flexibility and durability, representing a promising candidate for sensitive and robust CPL photodetectors. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 研究了手性Quasi-2D钙钛矿单晶（SCS），用于其圆偏振光（CPL）检测能力。准2D手性佩洛夫斯基酯，[（ R </ I> ）-β-MPA] <sub> 2 </ sub> MAPB. <sub> 2 </ sub> 一世 <sub> 7 </ sub> （（ R </ I> ）-β-MPa =（ R </ I> ） - （+） - β-甲基苯乙胺，MA =甲基铵），具有内在的手性和区分CPL光子的不同偏振态的能力。相应的准二维SCS CPL光电探测器表现出优异的检测性能。特别地，我们的设备响应性几乎比报告的2D PEROVSKITE CPL探测器高出一个数量级。调节薄膜的结晶动力学以促进其载体运输。具有均匀能量景观的平行定向的钙钛矿薄膜对于最大化载流子收集效率至关重要。光电探测器还具有出色的机械柔性和耐用性，代表敏感和鲁棒CPL光电探测器的有希望的候选者。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Lin&option=202" target="_blank" rel="nofollow">Wang Lin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xue Yongxiang&option=202" target="_blank" rel="nofollow">Xue Yongxiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cui Minghuan&option=202" target="_blank" rel="nofollow">Cui Minghuan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Yanmin&option=202" target="_blank" rel="nofollow">Huang Yanmin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Hongyu&option=202" target="_blank" rel="nofollow">Xu Hongyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qin Chaochao&option=202" target="_blank" rel="nofollow">Qin Chaochao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Jien&option=202" target="_blank" rel="nofollow">Yang Jien;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dai Haitao&option=202" target="_blank" rel="nofollow">Dai Haitao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yuan Mingjian&option=202" target="_blank" rel="nofollow">Yuan Mingjian;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education)Nankai UniversityTianjin 300071 P. R. China;</p> <p>Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparing TechnologyTianjin UniversityTianjin 300072 P. R. China;</p> <p>Henan Key Laboratory of Infrared Materials &</p> <p>Spectrum Measures and ApplicationsHenan Normal UniversityXinxiang 453007 P.R. China;</p> <p>Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education)Nankai UniversityTianjin 300071 P. R. China;</p> <p>Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education)Nankai UniversityTianjin 300071 P. R. China;</p> <p>Henan Key Laboratory of Infrared Materials &</p> <p>Spectrum Measures and ApplicationsHenan Normal UniversityXinxiang 453007 P.R. China;</p> <p>Henan Key Laboratory of Infrared Materials &</p> <p>Spectrum Measures and ApplicationsHenan Normal UniversityXinxiang 453007 P.R. China;</p> <p>Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparing TechnologyTianjin UniversityTianjin 300072 P. R. China;</p> <p>Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education)Nankai UniversityTianjin 300071 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=chiral perovskites&option=203" rel="nofollow">chiral perovskites;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=circular polarized light&option=203" rel="nofollow">circular polarized light;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=crystallization dynamics&option=203" rel="nofollow">crystallization dynamics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photodetector&option=203" rel="nofollow">photodetector;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=reduced-dimension perovskites&option=203" rel="nofollow">reduced-dimension perovskites;</a> </p> <div class="translation"> 机译：手性肝脏;圆形偏振光;结晶动力学;光电探测器;减数普罗夫斯基斯; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028161535.html">A Chiral Reduced‐Dimension Perovskite for an Efficient Flexible 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