Promoting the Electrocatalytic Performance of Noble Metal Aerogels by Ligand‐Directed Modulation

摘要

Abstract >Noble metal aerogels (NMAs) are an emerging class of porous materials. Embracing nano‐sized highly‐active noble metals and porous structures, they display unprecedented performance in diverse electrocatalytic processes. However, various impurities, particularly organic ligands, are often involved in the synthesis and remain in the corresponding products, hindering the investigation of the intrinsic electrocatalytic properties of NMAs. Here, starting from laser‐generated inorganic‐salt‐stabilized metal nanoparticles, various impurity‐free NMAs (Au, Pd, and Au‐Pd aerogels) were fabricated. In this light, we demonstrate not only the intrinsic electrocatalytic properties of NMAs, but also the prominent roles played by ligands in tuning electrocatalysis through modulating the electron density of catalysts. These findings may offer a new dimension to engineer and optimize the electrocatalytic performance for various NMAs and beyond. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >贵金属气凝胶（Nmas）是一种新兴的多孔材料。拥抱纳米大小的高活度贵金属和多孔结构，它们在不同的电催化过程中显示出前所未有的性能。然而，各种杂质，特别是有机配体通常涉及合成并留在相应的产品中，妨碍了NMA的内在电催化性质的研究。这里，从激光产生的无机盐稳定金属纳米颗粒开始，制造各种无杂质NMA（Au，Pd和Au-Pd Aerogels）。在这种光中，我们不仅展示了NMA的内在电催化性质，而且表明了配体通过调节催化剂的电子密度来调节电殖分析的突出角色。这些调查结果可以为工程师提供新的维度，并优化各种NMA和超越的电催化性能。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第14期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=aerogels&option=203" rel="nofollow">aerogels;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysis&option=203" rel="nofollow">electrocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=laser&option=203" rel="nofollow">laser;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ligand&option=203" rel="nofollow">ligand;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=noble metals&option=203" rel="nofollow">noble metals;</a> </p> <div class="translation"> 机译：气凝胶;电殖分析;激光;配体;贵金属; </div> </li> </ul> 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noble metals by either direct or indirect printing</a> <b>[P]</b> . <span> 外国专利：  CZ245299A3 </span> <span> . 2000-03-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：贵金属的制备及其通过直接或间接印刷由贵金属生产装饰体的用途 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130450869583.html">Preparation of noble metals and its use for producing ornamental bodies from noble metals by either direct or indirect printing</a> <b>[P]</b> . <span> 外国专利：  CZ9902452A3 </span> <span> . 2000-03-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：贵金属的制备及其通过直接或间接印刷由贵金属生产装饰体的用途 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130429251179.html">Single component precursor, useful e.g. to manufacture noble metal/titanium dioxide-composite material, comprises water-soluble titanium dioxide-complex with multidentate carboxylate containing ligand and water-soluble noble metal anion</a> <b>[P]</b> . <span> 外国专利：  DE102008011337A1 </span> <span> . 2009-09-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：单组分前体，有用的例如制备贵金属/二氧化钛复合材料，包括水溶性二氧化钛配合物，以及含有配体和水溶性贵金属阴离子的多齿羧酸盐 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" 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