Switching of Redox Properties Triggered by a Thermal Equilibrium between Closed‐Shell Folded and Open‐Shell Twisted Species

Ishigaki Yusuke; Hashimoto Takumi; Sugawara Kazuma; Suzuki Shuichi; Suzuki Takanori

摘要

Abstract >Thermally switchable redox properties have been reported to be due to a change in the spin state of newly designed overcrowded ethylenes, which can adopt closed‐shell folded and open‐shell twisted forms. In this study, tetrathienylanthraquinodimethane derivatives were designed to be in thermal equilibrium between a more stable folded form and less stable but more donating twisted diradical in solution, so that the oxidation potential can be controlled by heating/cooling. This is the first example of a switching of redox properties based on a thermally equilibrated twisted diradical, which can be more readily oxidized to the twisted dication. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> 据报道，据报道，由于新设计的新设计过度拥挤的乙烯的旋转状态的变化，可以采用封闭壳折叠和开壳捻捻形式的旋转状态的变化。在该研究中，Tethathienylthraquinodimodimodimodemone衍生物被设计为在更稳定的折叠形式和更稳定的稳定性中的热平衡，但在溶液中的扭曲扭曲，从而可以通过加热/冷却来控制氧化电位。这是基于热平衡的扭曲的Daradical的氧化还原性能切换的第一示例，这可以更容易地氧化成扭曲的DIRG。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共4页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ishigaki Yusuke&option=202" target="_blank" rel="nofollow">Ishigaki Yusuke;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hashimoto Takumi&option=202" target="_blank" rel="nofollow">Hashimoto Takumi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sugawara Kazuma&option=202" target="_blank" rel="nofollow">Sugawara Kazuma;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Suzuki Shuichi&option=202" target="_blank" rel="nofollow">Suzuki Shuichi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Suzuki Takanori&option=202" target="_blank" rel="nofollow">Suzuki Takanori;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryHokkaido UniversitySapporo 060-0810 Japan;</p> <p>Department of ChemistryHokkaido UniversitySapporo 060-0810 Japan;</p> <p>Department of ChemistryHokkaido UniversitySapporo 060-0810 Japan;</p> <p>Graduate School of Engineering ScienceOsaka UniversityOsaka 560-8531 Japan;</p> <p>Department of ChemistryHokkaido UniversitySapporo 060-0810 Japan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=cations&option=203" rel="nofollow">cations;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=overcrowded ethylenes&option=203" rel="nofollow">overcrowded ethylenes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=radicals&option=203" rel="nofollow">radicals;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=redox chemistry&option=203" rel="nofollow">redox chemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thermal equilibrium&option=203" rel="nofollow">thermal equilibrium;</a> </p> <div class="translation"> 机译：阳离子;过度拥挤的乙烯;自由基;氧化还原化学;热平衡; 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