Algae Extraction Controllable Delamination of Vanadium Carbide Nanosheets with Enhanced Near‐Infrared Photothermal Performance

Zada Shah; Dai Wenhao; Kai Zhang; Lu Huiting; Meng Xiangdan; Zhang Yiyi; Cheng Yaru; Yan Fang; Fu Pengcheng; Zhang Xueji; Dong Haifeng

摘要

Abstract > The two‐dimensional (2D) vanadium carbide (V <sub>2</sub> C) MXene has shown great potential as a photothermal agent (PTA) for photothermal therapy (PTT). However, the use of V <sub>2</sub> C in PTT is limited by the harsh synthesis condition and low photothermal conversion efficiency (PTCE). Herein, we report a completely different green delamination method using algae extraction to intercalate and delaminate V <sub>2</sub> AlC to produce mass V <sub>2</sub> C nanosheets (NSs) with a high yield (90?%). The resulting V <sub>2</sub> C NSs demonstrated good structural integrity and remarkably high absorption in near infrared (NIR) region with a PTCE as high as 48?%. Systemic in vitro and in vivo studies demonstrate that the V <sub>2</sub> C NSs can serve as efficient PTA for photoacoustic (PA) and magnetic resonance imaging (MRI)‐guided PTT of cancer. This work provides a cost‐effective, environment‐friendly, and high‐yielding disassembly approach of MAX, opening a new avenue to develop MXenes with desirable properties for a myriad of applications. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 二维（2D）碳化钒（V <sub> 2 </ sub> c）MXENE表现为光热疗法（PTT）的光热试剂（PTA）的潜力很大。但是，使用v <sub> 2 </ sub> C在PTT中受到严苛合成条件和低光热转换效率（PTCE）的限制。在此，我们通过藻类提取来报告一种完全不同的绿化分层方法，以嵌入和分层v <sub> 2 </ sub> ALC生产质量v <sub> 2 </ sub> C纳米蛋白酶（NSS）高产量（90？％）。由此产生的V. <sub> 2 </ sub> C NSS在近红外（NIR）区域中展示了良好的结构完整性，并且在近红外（NIR）区域具有显着高，PTCE高达48Ω％。体外系统和体内研究表明V <sub> 2 </ sub> C NSS可以用作光声（PA）和磁共振成像（MRI）导癌的磁共振成像（MRI）的高效PTA。这项工作提供了具有成本效益，环保的和高产的最大拆卸方法，开启了一个新的途径，为MXENES开发了具有无数应用程序的理想性质。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zada Shah&option=202" target="_blank" rel="nofollow">Zada Shah;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dai Wenhao&option=202" target="_blank" rel="nofollow">Dai Wenhao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kai Zhang&option=202" target="_blank" rel="nofollow">Kai Zhang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lu Huiting&option=202" target="_blank" rel="nofollow">Lu Huiting;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Meng Xiangdan&option=202" target="_blank" rel="nofollow">Meng Xiangdan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Yiyi&option=202" target="_blank" rel="nofollow">Zhang Yiyi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cheng Yaru&option=202" target="_blank" rel="nofollow">Cheng Yaru;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Fang&option=202" target="_blank" rel="nofollow">Yan Fang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fu Pengcheng&option=202" target="_blank" rel="nofollow">Fu Pengcheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xueji&option=202" target="_blank" rel="nofollow">Zhang Xueji;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dong Haifeng&option=202" target="_blank" rel="nofollow">Dong Haifeng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>School of Chemistry and Biological EngineeringUniversity of Science &</p> <p>Technology Beijing30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>State Key Laboratory of Marine Resource Utilization in South China Sea Hainan University58 Renmin Avenue Meilan District Haikou Hainan Province 570228 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> <p>Beijing Key Laboratory for Bioengineering and Sensing TechnologySchool of Chemistry and Biological Engineering30 Xueyuan Road Beijing 100083 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=algae extraction&option=203" rel="nofollow">algae extraction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=cancer&option=203" rel="nofollow">cancer;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=exfoliation&option=203" rel="nofollow">exfoliation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=MXene&option=203" rel="nofollow">MXene;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photothermal therapy&option=203" rel="nofollow">photothermal therapy;</a> </p> <div class="translation"> 机译：藻类萃取;癌症;剥离;MXENE;光热疗法; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028161347.html">Algae Extraction Controllable Delamination of Vanadium Carbide Nanosheets with Enhanced Near‐Infrared Photothermal Performance</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zada Shah&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zada Shah,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dai Wenhao&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dai Wenhao,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kai Zhang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Kai Zhang,</a> <a href="/journal-foreign-19011/" target="_blank" rel="nofollow" class="tuijian_authcolor">Angewandte Chemie .</a> <span>2020</span><span>,第16期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：近红外光热性能提高碳化钒纳米液的藻类萃取可控分层</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_applied-surface-science_thesis/0204113784609.html">Growth of self-aligned single-crystal vanadium carbide nanosheets with a controllable thickness on a unique staked metal substrate</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> </a> <a href="/journal-foreign-705/" target="_blank" rel="nofollow" class="tuijian_authcolor">Applied Surface Science .</a> <span>2020</span><span>,第Jana1期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在独特的金属桩基上生长可控制厚度的自对准单晶碳化钒纳米片</span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028188029.html">Plasmonic molybdenum oxide nanosheets supported silver nanocubes for enhanced near-infrared antibacterial activity: Synergism of photothermal effect, silver release and photocatalytic reactions</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yin Qiaoqiao&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yin Qiaoqiao,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tan Linxiang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Tan Linxiang,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lang Qingqing&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Lang Qingqing,</a> <a href="/journal-foreign-19279/" target="_blank" rel="nofollow" class="tuijian_authcolor">Applied Catalysis, B. 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