Radially Inwardly Aligned Hierarchical Porous Carbon for Ultra‐Long‐Life Lithium–Sulfur Batteries

Yu Zhisheng; Liu Menglan; Guo Daying; Wang Jiahui; Chen Xing; Li Jun; Jin Huile; Yang Zhi; Chen Xian; Wang Shun

摘要

Abstract >Rational design of hollow micro‐ and/or nano‐structured cathodes as sulfur hosts has potential for high‐performance lithium‐sulfur batteries. However, their further commercial application is hindered because infusing sulfur into hollow hosts is hard to control and the interactions between high loading sulfur and electrolyte are poor. Herein, we designed hierarchical porous hollow carbon nanospheres with radially inwardly aligned supporting ribs to mitigate these problems. Such a structure could aid the sulfur infusion and maximize sulfur utilization owing to the well‐ordered pore channels. This highly organized internal carbon skeleton can also enhance the electronic conductivity. The hollow carbon nanospheres with further nitrogen‐doping as the sulfur host material exhibit good capacity and excellent cycling performance (0.044?% capacity degradation per each cycle for 1000?cycles). </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P>作为硫宿主具有高性能锂 - 硫磺电池的空心微型和/或纳米结构阴极的理性设计。然而，他们的进一步商业应用受到阻碍，因为将硫注入空心主体是难以控制的，并且高负载硫和电解质之间的相互作用差。在此，我们设计了具有径向向内排列的支撑肋的分层多孔中空碳纳米，以减轻这些问题。这种结构可以帮助硫输注并最大限度地利用由于井有序的孔通道。这种高度组织的内碳骨架也可以增强电子电导率。具有进一步氮气掺杂的中空碳纳米球作为硫磺宿主材料表现出良好的容量和优异的循环性能（每个循环每周的容量降解0.044Ω·倍次）。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yu Zhisheng&option=202" target="_blank" rel="nofollow">Yu Zhisheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Menglan&option=202" target="_blank" rel="nofollow">Liu Menglan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Daying&option=202" target="_blank" rel="nofollow">Guo Daying;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Jiahui&option=202" target="_blank" rel="nofollow">Wang Jiahui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Xing&option=202" target="_blank" rel="nofollow">Chen Xing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Jun&option=202" target="_blank" rel="nofollow">Li Jun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jin Huile&option=202" target="_blank" rel="nofollow">Jin Huile;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Zhi&option=202" target="_blank" rel="nofollow">Yang Zhi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Xian&option=202" target="_blank" rel="nofollow">Chen Xian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Shun&option=202" target="_blank" rel="nofollow">Wang Shun;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> <p>Key Laboratory of Carbon Materials of Zhejiang ProvinceWenzhou UniversityWenzhou 325035 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-sulfur batteries&option=203" rel="nofollow">lithium-sulfur batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=N-doped carbon nanospheres&option=203" rel="nofollow">N-doped carbon nanospheres;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hierarchical porous carbon&option=203" rel="nofollow">hierarchical porous carbon;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=tailored interior structure&option=203" rel="nofollow">tailored interior structure;</a> </p> <div class="translation"> 机译：锂 - 硫磺电池;正掺杂的碳纳米球;等级多孔碳;量身定制的室内结构; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028161276.html">Radially Inwardly Aligned Hierarchical Porous Carbon for Ultra‐Long‐Life Lithium–Sulfur Batteries</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yu Zhisheng&option=202" 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</div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_computer-measurement-control_thesis/0201242100110.html">锂-亚硫酰氯电池储存寿命研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=叶浩亮&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 叶浩亮</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李飞&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,李飞</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王松林&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王松林</a> <span> <a href="/journal-cn-8916/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 计算机测量与控制 </a> </span> <span> . 2017</span><span>,第005期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-8041_thesis/020222065847.html">智能电表用锂/亚硫酰氯电池加速寿命试验</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=祝媛&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 祝媛</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张福义&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张福义</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=袁中直&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,袁中直</a> <span> <a href="/conference-cn-8041/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 全国电工仪器仪表标准化技术委员会第四届五次全体委员会议暨2012第二十五届电磁测量技术、标准、产品国际研讨及展会 </a> <span> <span> . 2012</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020312287484.html">多孔碳材料在高比能锂硫、锂硒电池中的应用</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=吴超&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 吴超</a> <span> . 2015</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120107128925.html">用于锂-硫电池的多孔碳中间层</a> <b>[P]</b> . <span> 中国专利： CN104620416A </span> <span> . 2015-05-13</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120103728398.html">用于改善锂硫二次电池的寿命特性和充电速度的方法</a> <b>[P]</b> . <span> 中国专利： CN111052492A </span> <span> . 2020-04-21</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130499881709.html">Porous carbon material, method for producing porous carbon material, composite, method for manufacturing composite, positive electrode for lithium-sulfur battery, and lithium-sulfur battery</a> <b>[P]</b> . <span> 外国专利：  JP2021066618A </span> <span> . 2021-04-30</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：多孔碳材料，生产多孔碳材料，复合材料，制造复合材料的方法，用于锂 - 硫电池的正电极，以及锂 - 硫电池 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130408745332.html">Hierarchical architecture with nanosized metal oxide and porous graphene for lithium ion battery anode with ultra-fast charge/discharge rate and extremely robust cycle life using thereof</a> <b>[P]</b> . <span> 外国专利：  KR20170022747A </span> <span> . 2017-03-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于锂离子电池阳极的纳米级金属氧化物和多孔石墨烯的分层体系结构，具有超快的充电/放电速率和使用其的超强循环寿命 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130408589929.html">Hierarchical architecture with nanosized metal oxide and porous graphene for lithium ion battery anode with ultra-fast charge/discharge rate and extremely robust cycle life using thereof</a> <b>[P]</b> . <span> 外国专利：  KR101745449B1 </span> <span> . 2017-06-12</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于锂离子电池阳极的纳米级金属氧化物和多孔石墨烯的分层体系结构，具有超快的充电/放电速率和使用其的超强循环寿命 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704028161276','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" 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