Spontaneous Synthesis of Silver‐Nanoparticle‐Decorated Transition‐Metal Hydroxides for Enhanced Oxygen Evolution Reaction

Zhang Zhao; Li Xiaopeng; Zhong Cheng; Zhao Naiqin; Deng Yida; Han Xiaopeng; Hu Wenbin

摘要

Abstract > The fabrication of metal‐supported hybrid structures with enhanced properties typically requires external energy input, such as pyrolysis, photolysis, and electrodeposition. In this study, silver‐nanoparticle‐decorated transition‐metal hydroxide (TMH) composites were synthesized by an approach based on a spontaneous redox reaction (SRR) at room temperature. The SRR between silver ions and TMH provides a simple and facile route to establish effective and stable heterostructures that can enhance the oxygen evolution reaction (OER) activity. Ag@Co(OH) <sub> x </sub> grown on carbon cloth exhibits outstanding OER activity and durability, even superior to IrO <sub>2</sub> and many previously reported OER electrocatalysts. Experimental and theoretical analysis demonstrates that the strong electronic interaction between Ag and Co(OH) <sub>2</sub> activates the silver clusters as catalytically OER active sites, effectively optimizing the binding energies with reacted intermediates and facilitating the OER kinetics. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 具有增强特性的金属支持的混合结构的制造通常需要外部能量输入，例如热解，光解和电沉积。在该研究中，通过在室温下基于自发的氧化还原反应（SRR）的方法，通过基于自发的氧化还原反应（SRR）来合成银纳米粒子装饰的过渡金属氢氧化物（TMH）复合材料。银离子和TMH之间的SRR提供了一种简单且容易的途径，以建立有效且稳定的异质结构，可以增强氧气进化反应（OER）活性。 ag @ co（哦） <sub> x </ i> </ sub> 在碳布上成长，展示出色的OER活动和耐用性，甚至优于IRO <sub> 2 </ sub> 并且许多先前报告的oer电催化剂。实验和理论分析表明，AG和CO（OH）之间的强电子互动 <sub> 2 </ sub> 将银簇作为催化陶氏活性位点激活，有效地优化与反应中间体的结合能量，并促进oer动力学。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第18期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Zhao&option=202" target="_blank" rel="nofollow">Zhang Zhao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Xiaopeng&option=202" target="_blank" rel="nofollow">Li Xiaopeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhong Cheng&option=202" target="_blank" rel="nofollow">Zhong Cheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Naiqin&option=202" target="_blank" rel="nofollow">Zhao Naiqin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Deng Yida&option=202" target="_blank" rel="nofollow">Deng Yida;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Han Xiaopeng&option=202" target="_blank" rel="nofollow">Han Xiaopeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hu Wenbin&option=202" target="_blank" rel="nofollow">Hu Wenbin;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin UniversityTianjin 300350 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydroxides&option=203" rel="nofollow">hydroxides;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanocomposites&option=203" rel="nofollow">nanocomposites;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen evolution&option=203" rel="nofollow">oxygen evolution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=silver&option=203" rel="nofollow">silver;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=spontaneous redox reaction&option=203" rel="nofollow">spontaneous redox reaction;</a> </p> <div class="translation"> 机译：氢氧化物;纳米复合材料;氧气进化;银;自发氧化还原反应; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028160950.html">Spontaneous Synthesis of Silver‐Nanoparticle‐Decorated Transition‐Metal Hydroxides for Enhanced Oxygen Evolution 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