Coverage‐Controlled Superstructures of C3‐Symmetric Molecules: Honeycomb versus Hexagonal Tiling

Jasper‐T?nnies Torben; Gruber Manuel; Ulrich Sandra; Herges Rainer; Berndt Richard

摘要

Abstract > The competition between honeycomb and hexagonal tiling of molecular units can lead to large honeycomb superstructures on surfaces. Such superstructures exhibit pores that may be used as 2D templates for functional guest molecules. Honeycomb superstructures of molecules that comprise a C <sub>3</sub> symmetric platform on Au(111) and Ag(111) surfaces are presented. The superstructures cover nearly mesoscopic areas with unit cells containing up to 3000 molecules, more than an order of magnitude larger than previously reported. The unit cell size may be controlled by the coverage. A fairly general model was developed to describe the energetics of honeycomb superstructures built from C <sub>3</sub> symmetric units. Based on three parameters that characterize two competing bonding arrangements, the model is consistent with the present experimental data and also reproduces various published results. The model identifies the relevant driving force, mostly related to geometric aspects, of the pattern formation. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 分子单元的蜂窝和六边形平铺之间的竞争可能导致表面上的大蜂窝上部结构。这种上层建筑表现出可用作功能性客体分子的2D模板的孔。包含C的蜂窝上部结构的分子 <sub> 3 </ sub> 呈现AU（111）和AG（111）表面的对称平台。上部结构覆盖具有含有多达3000个分子的单位细胞的几乎是瞳孔细胞，比以前报道的大于100多个数量级。单元电池大小可以由覆盖范围控制。开发了一个相当一般的模型来描述由蜂窝上层建筑的能量学 c </ i> <sub> 3 </ sub> 对称单位。基于三个参数，该参数表征了两个竞争绑定装置，该模型与本实验数据一致，同样再现各种公开的结果。该模型识别模式形成的相关驱动力，主要与几何方面相关。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第18期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jasper‐T?nnies Torben&option=202" target="_blank" rel="nofollow">Jasper‐T?nnies Torben;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gruber Manuel&option=202" target="_blank" rel="nofollow">Gruber Manuel;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ulrich Sandra&option=202" target="_blank" rel="nofollow">Ulrich Sandra;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Herges Rainer&option=202" target="_blank" rel="nofollow">Herges Rainer;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Berndt Richard&option=202" target="_blank" rel="nofollow">Berndt Richard;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Institut für Experimentelle und Angewandte PhysikChristian-Albrechts-Universit?t24098 Kiel Germany;</p> <p>Institut für Experimentelle und Angewandte PhysikChristian-Albrechts-Universit?t24098 Kiel Germany;</p> <p>Otto-Diels-Institut für Organische ChemieChristian-Albrechts-Universit?t24098 Kiel Germany;</p> <p>Otto-Diels-Institut für Organische ChemieChristian-Albrechts-Universit?t24098 Kiel Germany;</p> <p>Institut für Experimentelle und Angewandte PhysikChristian-Albrechts-Universit?t24098 Kiel Germany;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=C3-symmetric molecules&option=203" rel="nofollow">C3-symmetric molecules;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=coverage control&option=203" rel="nofollow">coverage control;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=honeycomb superstructure&option=203" rel="nofollow">honeycomb superstructure;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=molecular tiling model&option=203" rel="nofollow">molecular tiling model;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=scanning tunneling microscopy&option=203" rel="nofollow">scanning tunneling microscopy;</a> </p> <div class="translation"> 机译：C3-对称分子;覆盖控制;蜂窝上部结构;分子平铺模型;扫描隧道显微镜; 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href="/patent-detail/061203580307.html">一种蜂窝六边形钛硅分子筛及其制备方法和用途</a> <b>[P]</b> . <span> 中国专利： CN107265474B </span> <span> . 2019.12.20</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120109745344.html">一种蜂窝六边形钛硅分子筛及其制备方法和用途</a> <b>[P]</b> . <span> 中国专利： CN107265474A </span> <span> . 2017-10-20</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130474172192.html">series of no.two tile shaped accostabili between them, one of which has a shape symmetrical to tozzetto quadrilobata has edges shaped to curly brace.and the other is hexagonal with two sides opposing each other having a shape complementary to that of the edges of tozzetto.</a> <b>[P]</b> . <span> 外国专利：  IT8434802V0 </span> <span> . 1984-01-09</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：它们之间有一系列的两个砖瓦状可口齿形状，其中一个形状与四边形的托泽特对称，边的形状呈花括号状，另一个为六边形，两侧彼此相对，形状与托塞特的边缘互补。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130401562138.html">SYMMETRIC CONTROL OF AN ASYMMETRIC AC MOTOR VIA A FLUX REGULATOR OPERATING BASED ON A TARGETED TIME CONSTANT VERSUS SAMPLING PERIOD RATIO</a> <b>[P]</b> . <span> 外国专利：  US2020127588A1 </span> <span> . 2020-04-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：基于目标时间常数与采样周期比率的磁通调节器操作的非对称交流电动机的对称控制 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130431271153.html">HEXAGONAL-CELL HONEYCOMB CATALYST BODY, AND EXHAUST EMISSION CONTROL SYSTEM USING THE SAME</a> <b>[P]</b> . <span> 外国专利：  JP2009011976A </span> <span> . 2009-01-22</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: 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