Design of Complex Solid‐Solution Electrocatalysts by Correlating Configuration, Adsorption Energy Distribution Patterns, and Activity Curves

摘要

Abstract >Complex solid‐solution electrocatalysts (also referred to as high‐entropy alloy) are gaining increasing interest owing to their promising properties which were only recently discovered. With the capability of forming complex single‐phase solid solutions from five or more constituents, they offer unique capabilities of fine‐tuning adsorption energies. However, the elemental complexity within the crystal structure and its effect on electrocatalytic properties is poorly understood. We discuss how addition or replacement of elements affect the adsorption energy distribution pattern and how this impacts the shape and activity of catalytic response curves. We highlight the implications of these conceptual findings on improved screening of new catalyst configurations and illustrate this strategy based on the discovery and experimental evaluation of several highly active complex solid solution nanoparticle catalysts for the oxygen reduction reaction in alkaline media. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >复合物固体溶液电催化剂（也称为高熵合金）由于最近发现的有希望的性质而言，越来越多的利益。通过从五种或更多种成分形成复杂的单相固体溶液的能力，它们提供了微调吸附能的独特能力。然而，晶体结构内的元素复杂性及其对电催化性质的影响是较差的。我们讨论元素的添加或更换如何影响吸附能量分布模式以及这种情况如何影响催化反应曲线的形状和活性。我们突出了这些概念发现对新型催化剂配置的改善筛选的影响，并根据碱性介质中的氧还原反应的氧还原反应的发现和实验评价来说明该策略。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第14期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=catalyst screening&option=203" rel="nofollow">catalyst screening;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysis&option=203" rel="nofollow">electrocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=high-entropy alloys&option=203" rel="nofollow">high-entropy alloys;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=intrinsic activity&option=203" rel="nofollow">intrinsic activity;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen reduction reaction (ORR)&option=203" rel="nofollow">oxygen reduction reaction (ORR);</a> </p> <div class="translation"> 机译：催化剂筛选;电催化;高熵合金;内在活动;氧还原反应（ORR）; 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<b>[P]</b> . <span> 中国专利： CN110657312B </span> <span> . 2021.05.25</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120103389524.html">基于能量平衡的紧凑型恒力弹簧支吊架凸轮曲线设计方法</a> <b>[P]</b> . <span> 中国专利： CN110657312A </span> <span> . 2020-01-07</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130443027543.html">In metal genus of specification the solution constituent and the solution constituent for rare earth super-conductivity film production which include the metal complex which configuration it could point the ligand of specification, the non crystal solid of the specific metal complex, in metal genus of specification production manner of the solution which includes the metal complex which configuration it could point the ligand of specification, production manner of the solution for rare earth super-conductivity film production, and production manner of the super-conductivity thin film.</a> <b>[P]</b> . <span> 外国专利：  JP3548802B2 </span> <span> . 2004-07-28</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在规范的金属属中，规范成分的金属属中的溶液成分和用于稀土超导膜生产的溶液成分包括配置可以指向规范的配体，特定金属络合物的非晶态的金属配合物的结构包括金属配合物的溶液的生产方式，其结构可以指明规格的配体，稀土超导膜生产用溶液的生产方式以及超导薄膜的生产方式。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130443027544.html">In metal genus of specification the solution constituent and the solution constituent for rare earth super-conductivity film production which include the metal complex which configuration it could point the ligand of specification, the non crystal solid of the specific metal complex, in metal genus of specification production manner of the solution which includes the metal complex which configuration it could point the ligand of specification, production manner of the solution for rare earth super-conductivity film production, and formation manner of the super-conductivity thin film.</a> <b>[P]</b> . <span> 外国专利：  JP3548801B2 </span> <span> . 2004-07-28</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在规范的金属属中，规范成分的金属属中的溶液成分和用于稀土超导膜生产的溶液成分包括配置可以指向规范的配体，特定金属络合物的非晶态的金属配合物的结构溶液的生产方式包括可以指定规格的配体的金属配合物，稀土超导膜生产用溶液的生产方式以及超导薄膜的形成方式。 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130440301064.html">METHOD FOR ESTIMATING REMAINING FILM THICKNESS DISTRIBUTION, METHOD FOR DESIGNING PATTERNING MASK USING THE METHOD FOR ESTIMATING REMAINING FILM THICKNESS DISTRIBUTION, AND METHOD FOR MANUFACTURING SEMICONDUCTOR DEVICES BY USING PATTERNING MASK DESIGNED BY USING THE METHOD FOR ESTIMATING REMAINING FILM THICKNESS DISTRIBUTION</a> <b>[P]</b> . <span> 外国专利：  US6905966B2 </span> <span> . 2005-06-14</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：估计剩余膜厚分布的方法，使用估计剩余膜厚分布的方法设计图案的方法，以及通过使用通过估计膜厚的方法设计的图案的掩模来制造半导体器件的方法 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704028160744','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p 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