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Observing the Angular Distribution of Raman Scattered Fields

机译:观察拉曼散射场的角分布

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In conventional optical spectroscopy, lenses are used to focus light on the sample and to collect light scattered from the sample. Focusing increases the signal intensity, but it amounts to angular (k-space) averaging and leads to information loss. In this issue of ACS Nano, Budde and collaborators record radiation patterns of Raman scattering from a single layer of graphene, revealing the angular distribution of the scattered field. The authors show that the radiation patterns render the spatial symmetry of vibrational modes. Furthermore, their results demonstrate that depolarization effects occurring in the focal region must be taken into account for proper interpretation of Raman intensities. We outline here the working principle of this new approach and discuss future applications for studies of graphene and other low-dimensional systems.
机译:在常规的光谱学中,透镜用于将光聚焦在样品上并收集从样品散射的光。聚焦会增加信号强度,但会导致角度(k空间)平均,并导致信息丢失。在本期ACS Nano中,Budde和合作者记录了来自单层石墨烯的拉曼散射的辐射图,揭示了散射场的角分布。作者表明,辐射图呈现出振动模态的空间对称性。此外,他们的结果表明,对于拉曼强度的正确解释,必须考虑在焦点区域发生的去极化效应。我们在这里概述了这种新方法的工作原理,并讨论了石墨烯和其他低维系统研究的未来应用。

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