Near Equilibrium        <sup >1313        C?        <sup >1818        O Bonding During Inorganic Calcite Precipitation Under Chemo‐Stat Conditions

Levitt Nicholas P.; Eiler John M.; Romanek Christopher S.; Beard Brian L.; Xu Huifang; Johnson Clark M.

摘要

Abstract > We report results of 13 C/ 12 C, 18 O/ 16 O, and 13 C? 18 O “clumped” isotope analyses from a series of calcite precipitation experiments from aqueous solutions under laboratory conditions. Chemo‐stat precipitation experiments were performed to synthetically form calcite from aqueous solution onto 43 Ca‐labeled calcite seed crystals. Formation rate was controlled during the experiments to investigate the effect of precipitation rate and temperature on 13 C? 18 O bonding in calcite, where rates ranged from 10 ?6.88 to 10 ?8.20 mol m ?2 s ?1 at three temperatures (10, 20, and 30°C). No relation was observed between precipitation rate and 13 C? 18 O bonding proportion over the range of precipitation rates used. The relation between Δ <sub>47</sub> and temperature produced?was comparable to calibration studies which report a relatively high sensitivity of 13 C? 18 O bonding to temperature?over the range investigated. Comparing solution conditions across multiple experimental data sets indicates an inverse relation between saturation state and 13 C? 18 O bonding, where high super‐saturation conditions are likely to be furthest from equilibrium 13 C? 18 O partitioning. Carbon fractionation between calcite and <mat:math display="inline" altimg="urn:x-wiley:15252027:media:ggge21521:ggge21521-math-1021" wiley:location="equation/ggge21521-math-1021.png"> <mat:mrow> <mat:msubsup> <mat:mtext>HCO</mat:mtext> <mat:mrow> <mat:mn>3</mat:mn> <mat:mo>(</mat:mo> <mat:mtext>aq</mat:mtext> <mat:mo>)</mat:mo> </mat:mrow> <mat:mo>?</mat:mo> </mat:msubsup> </mat:mrow> </mat:math> was found to be a temperature independent value of +1.6‰. The temperature‐dependent calcite‐water 18 O/ 16 O fractionation relation determined in this study is slightly different (larger <mat:math display="inline" altimg="urn:x-wiley:15252027:media:ggge21521:ggge21521-math-1020" wiley:location="equation/ggge21521-math-1020.png"> <mat:mrow> <mat:msub> <mat:mrow> <mat:mo>α</mat:mo> </mat:mrow> <mat:mrow> <mat:mrow> <mat:mtext>calcite</mat:mtext> <mat:mo>‐</mat:mo> <mat:msub> <mat:mi mathvariant="normal">H</mat:mi> <mat:mn>2</mat:mn> </mat:msub> <mat:mi mathvariant="normal">O</mat:mi> </mat:mrow> </mat:mrow> </mat:msub> </mat:mrow> </mat:math> value) than those measured in several previous investigations. Significantly, we observe a dependence of the 18 O/ 16 O isotope fractionation factor on growth rate. Taken together, these findings suggest carbonate growth in our experiments approached equilibrium more closely than previous experiments of this type, y </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“main”> <标题类型=“main”>抽象</ title> > 我们报告结果 13 </ sup> C/ 12 </ sup> C， 18 </ sup> o / 16 </ sup> o和 13 </ sup> C？ 18 </ sup> O“Clumped”同位素从实验室条件下的水溶液中的一系列方解石沉淀实验分析。通过水溶液合成形成化学统计沉淀实验 43 </ sup> Ca-标记的方解石种子晶体。在实验期间控制形成速率，以研究降水速率和温度的影响 13 </ sup> C？ 18 </ sup> o在方解石中键合，其中速率范围为10 ？6.88 </ sup> 到10. ？8.20 </ sup> 摩尔米？2 </ sup> S. ？1 </ sup> 在三个温度（10,20和30°C）。降水率和降水率之间没有关系 13 </ sup> C？ 18 </ sup> o在所用沉淀速率范围内粘合比例。 δ之间的关系 <sub> 47 </ sub> 产生的温度伴有？与校准研究相当，报告的敏感性相对较高 13 </ sup> C？ 18 </ sup> o将温度粘合？在调查范围内。比较多个实验数据集的解决方案条件指示饱和状态和饱和状态之间的反向关系 13 </ sup> C？ 18 </ sup> o键合，其中高超饱和条件可能从平衡中最远 13 </ sup> C？ 18 </ sup> o分区。方解石之间的碳分级和 <mat：数学显示=“内联”Altimg =“URN：X-Wiley：15252027：媒体：GGGE21521：GGGE21521-Math-1021”Wiley：Location =“等式/ GGGE21521-Math-1021.png”> <MAT：MROW> <mat：msubsup> <mat：mtext> hco </ mat：mtext> <MAT：MROW> <MAT：MN> 3 </ MAT：MN> <mat：mo>（</ mat：mo> <mat：mtext> aq </ mat：mtext> <mat：mo>）</ mat：mo> </ mat：MROW> <mat：mo>？</ mat：mo> </ mat：msubsup> </ mat：MROW> </ mat：math> 被发现是温度独立值+ 1.6‰。温度依赖性方解石水 18 </ sup> o / 16 </ sup> 在本研究中确定的分馏关系略有不同（更大 <mat：数学显示=“内联”Altimg =“URN：X-Wiley：15252027：GGGE21521：GGGE21521-Math-1020”Wiley：Location =“等式/ GGGE21521-Math-1020.png”> <MAT：MROW> <mat：msub> <MAT：MROW> <mat：mo>α</ mat：mo> </ mat：MROW> <MAT：MROW> <MAT：MROW> <mat：mtext>方解石</ mat：mtext> <mat：mo> - </ mat：mo> <mat：msub> <mat：mi mathvariant =“正常”> h </ mat：mi> <MAT：MN> 2 </ MAT：MN> </ mat：msub> <MAT：MI Mathvariant =“正常”> O </ MAT：MI> </ mat：MROW> </ mat：MROW> </ mat：msub> </ mat：MROW> </ mat：math> 价值比在几个先前的调查中测量的价值。显着，我们观察到的依赖 18 </ sup> o / 16 </ sup> o同位素分级对生长速率的分馏因子。在一起，这些研究结果表明我们的实验中的碳酸盐生长接近平衡比以前的这种类型的实验更紧密 </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23285/'>《Geochemistry, geophysics, geosystems》</a> <b style="margin: 0 2px;">|</b><span>2018年第3期</span><b style="margin: 0 2px;">|</b><span>共20页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Levitt Nicholas P.&option=202" target="_blank" rel="nofollow">Levitt Nicholas P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Eiler John M.&option=202" target="_blank" rel="nofollow">Eiler John M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Romanek Christopher S.&option=202" target="_blank" rel="nofollow">Romanek Christopher S.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Beard Brian L.&option=202" target="_blank" rel="nofollow">Beard Brian L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Huifang&option=202" target="_blank" rel="nofollow">Xu Huifang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Johnson Clark M.&option=202" target="_blank" rel="nofollow">Johnson Clark M.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>NASA Astrobiology Institute and Department of GeoscienceUniversity of Wisconsin‐MadisonMadison Wisconsin USA;</p> <p>NASA Astrobiology Institute and Geological and Planetary SciencesCalifornia Institute of TechnologyPasadena California USA;</p> <p>NASA Astrobiology Institute and Department of Earth and Environmental SciencesFurman UniversityGreenville South Carolina USA;</p> <p>NASA Astrobiology Institute and Department of GeoscienceUniversity of Wisconsin‐MadisonMadison Wisconsin USA;</p> <p>NASA Astrobiology Institute and Department of GeoscienceUniversity of Wisconsin‐MadisonMadison Wisconsin USA;</p> <p>NASA Astrobiology Institute and Department of GeoscienceUniversity of Wisconsin‐MadisonMadison Wisconsin USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=clumped isotopes&option=203" rel="nofollow">clumped isotopes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon&option=203" rel="nofollow">carbon;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen&option=203" rel="nofollow">oxygen;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=calcite&option=203" rel="nofollow">calcite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=isotope fractionation&option=203" rel="nofollow">isotope fractionation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=chemo‐stat&option=203" rel="nofollow">chemo‐stat;</a> </p> <div class="translation"> 机译：团块同位素;碳;氧;方解石;同位素分馏;化学统计; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023360793.html">Near Equilibrium <sup >1313 C? <sup >1818 O Bonding During Inorganic Calcite Precipitation Under Chemo‐Stat Conditions</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Levitt Nicholas P.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Levitt Nicholas P.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Eiler John M.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Eiler John M.,</a> <a 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Near Equilibrium 1313 C? 1818 O Bonding During Inorganic Calcite Precipitation Under Chemo‐Stat Conditions

摘要

Near Equilibrium ^{1313 C? ^{1818 O Bonding During Inorganic Calcite Precipitation Under Chemo‐Stat Conditions}}