Constraining the Fluid History of a CO        <sub >2</sub>2        ‐H        <sub >2</sub>2        S Reservoir: Insights From Stable Isotopes, REE, and Fluid Inclusion Microthermometry

Zwahlen Carmen; Hollis Cathy; Lawson Michael; Becker Stephen P.; Boyce Adrian; Zhou Zheng; Holland Greg

摘要

Abstract > Reservoirs that host CO <sub>2</sub> ‐H <sub>2</sub> S‐bearing gases provide a key insight into crustal redox reactions such as thermochemical sulfate reduction (TSR). Despite this, there remains a poor understanding of the extent, duration, and the factors limiting this process on a reservoir scale. Here we show how a combination of petrography, fluid inclusion, rare earth element (REE), and carbon (δ 13 C), oxygen (δ 18 O), and sulfur (δ 34 S) stable isotope data can disentangle the fluid history of the world's largest CO <sub>2</sub> accumulation, the LaBarge Field in Wyoming, USA. The carbonate‐hosted LaBarge Field was charged with oil around 80?Ma ago, which together with nodular anhydrite represent the reactants for TSR. The nodules exhibit two distinct trends of evolution in δ 13 C with both δ 34 S and δ 18 O that may be coupled to two different processes. The first trend was interpreted to reflect the coupled dissolution of anhydrite and reduction to elemental sulfur and the oxidation of organic compounds and associated precipitation of calcite during TSR. In contrast, the second trend was interpreted to be the result of the hydrothermal CO <sub>2</sub> influx after the cessation of TSR. In addition, mass balance calculations were performed to estimate an approximate TSR reaction duration of 80?ka and to identify the availability of organic compounds as the limiting factor of the TSR process. Such an approach provides a tool for the prediction of TSR occurrence elsewhere and advancing our understanding of crustal fluid interactions. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 水库主机CO <sub> 2 </ sub> -H <sub> 2 </ sub> S-轴承气体提供密钥洞察地壳的氧化还原反应，例如硫酸热化学还原（TSR）。尽管如此，仍然存在的范围内，持续时间的差的理解，并限制在一个水库规模此过程的因素。在这里，我们展示了如何岩石学，流体包裹体，稀土元素（REE）和碳（δ组合 13 </ sup> C），氧（δ 18 </ sup> O）和硫（δ 34 </ sup> S）稳定同位素数据可以解开世界上最大的二氧化碳的流体历史 <sub> 2 </ sub> 积累，LaBarge公司实地美国怀俄明州。碳酸盐托管LaBarge公司现场被控油约80？马前，与结节性硬石膏结合，表示反应物TSR。结节表现出δ进化的两种截然不同的发展趋势 13 </ sup> c用δ 34 </ sup> S和δ 18 </ sup> 但愿可以耦合到两个不同的过程。第一种趋势是解释为反映硬石膏和还原为元素硫TSR时的耦合溶解和有机化合物的氧化和方解石的相关联的沉淀。与此相反，第二个趋势被解释为水热CO的结果 <sub> 2 </ sub> TSR停止后涌入。另外，进行质量平衡计算来估算的80？KA近似TSR反应持续时间，并确定作为TSR过程的限制因素的有机化合物的可用性。这种方法提供了TSR发生在其他地方，并推进我们的地壳流体相互作用的了解的预测工具。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23285/'>《Geochemistry, geophysics, geosystems》</a> <b style="margin: 0 2px;">|</b><span>2019年第1期</span><b style="margin: 0 2px;">|</b><span>共24页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zwahlen Carmen&option=202" target="_blank" rel="nofollow">Zwahlen Carmen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hollis Cathy&option=202" target="_blank" rel="nofollow">Hollis Cathy;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lawson Michael&option=202" target="_blank" rel="nofollow">Lawson Michael;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Becker Stephen P.&option=202" target="_blank" rel="nofollow">Becker Stephen P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Boyce Adrian&option=202" target="_blank" rel="nofollow">Boyce Adrian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhou Zheng&option=202" target="_blank" rel="nofollow">Zhou Zheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Holland Greg&option=202" target="_blank" rel="nofollow">Holland Greg;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>The University of ManchesterManchester UK;</p> <p>The University of ManchesterManchester UK;</p> <p>ExxonMobil Upstream Research CompanySpring TX USA;</p> <p>ExxonMobil Upstream Research CompanySpring TX USA;</p> <p>Scottish Universities Environmental Research Centre (SUERC)East Kilbride UK;</p> <p>Lancaster Environment CentreLancaster UniversityLancaster UK;</p> <p>The University of ManchesterManchester UK;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=CO 2 reservoir&option=203" rel="nofollow">CO 2 reservoir;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=stable isotopes&option=203" rel="nofollow">stable isotopes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon sequestration&option=203" rel="nofollow">carbon sequestration;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbonate associated sulfate&option=203" rel="nofollow">carbonate associated sulfate;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=calcite nodules&option=203" rel="nofollow">calcite nodules;</a> </p> <div class="translation"> 机译：二氧化碳储层;稳定同位素;碳封存;碳酸酯相关硫酸盐;方解石结节; 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Constraining the Fluid History of a CO 22 ‐H 22 S Reservoir: Insights From Stable Isotopes, REE, and Fluid Inclusion Microthermometry

摘要

Constraining the Fluid History of a CO ₂2 ‐H ₂2 S Reservoir: Insights From Stable Isotopes, REE, and Fluid Inclusion Microthermometry