Improved Performance of Thick Films Based Binary and Ternary Bulk Heterojunction Organic Photovoltaic Devices Incorporated with Electrospinning Processed Nanofibers

Huang He Jun‐ning; Nan Hui Rong; Yang Ying Guo; Gao Xing Yu; Chen Fei; Chen Zhi‐Kuan

摘要

Abstract > Nanofibers (average diameter of ≈150–160 nm) consisting of both binary and ternary bulk heterojunction organic photovoltaic (BHJ‐OPV) donor‐acceptor pairs poly(3‐hexylthiophene):phenyl‐C61‐butyric acid methyl ester (P3HT:PC <sub>61</sub> BM) and (P3HT/PTB7:PC <sub>61</sub> BM) are produced in a coaxial electrospinning process. Thick (≈260 nm) BHJ‐OPV devices are fabricated by incorporating the nanofibers. Compared to thin (140 nm) P3HT:PC <sub>61</sub> BM binary devices, thick devices with P3HT:PC <sub>61</sub> BM nanofibers achieve an improved performance, i.e., an improvement from 65.15 to 73.24% in filling factor (FF), from 3.32 to 4.71% in power conversion efficiency (PCE), and from 8.51 to 11.09 mA cm ?2 in short‐circuit current density ( J <sub>sc</sub> ); while compared to thin P3HT/PTB7:PC <sub>61</sub> BM ternary devices, thick devices with P3HT/PTB7:PC <sub>61</sub> BM nanofibers show an improvement from 5.1 to 5.68% in PCE, from 12.51 to 14.74 mA cm ?2 in J <sub>sc</sub> , and a decrease from 66.83 to 63.55% in FF. The improved performance is attributed to an enhanced optical absorption induced by prolonged light absorption path due to scattering from nanofibers, a favorable nanomorphology with optimum crystallinity of P3HT/PTB7 and their good mixing with PC <sub>61</sub> BM, as well as an increased in‐plane alignment of P3HT and PTB7 polymer chains for efficient exciton dissociation and carrier extraction, and improved charge transport in the vertical direction. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 纳米纤维（平均直径为≈150-160nm），由二进制和三元散装异质结有机光伏（BHJ-OPV）供体对聚（3-己基噻吩）：苯基-C61-丁酸甲酯（P3HT：PC <sub> 61 </ sub> BM）和（P3HT / PTB7：PC <sub> 61 </ sub> BM）在同轴电纺丝过程中生产。厚（≈260nm）通过掺入纳米纤维来制造BHJ-OPV器件。与薄（140nm）p3ht：pc相比 <sub> 61 </ sub> BM二进制设备，带P3HT的厚设备：PC <sub> 61 </ sub> BM纳米纤维获得的性能提高，即填充因子（FF）的65.15至73.24％的改善，从电力转换效率（PCE）的3.32％至4.71％，以及8.51至11.09 mA cm ？2 </ sup> 在短路电流密度（ j </ i> <sub> sc </ sub> ）;与薄P3HT / PTB7：PC相比 <sub> 61 </ sub> BM三元设备，带P3HT / PTB7：PC的厚设备 <sub> 61 </ sub> BM纳米纤维在PCE中的改善从12.51到14.74 mA厘米的5.1％到5.68％？2 </ sup> 在 j </ i> <sub> sc </ sub> ，在FF中减少66.83至63.55％。提高的性能归因于由于沿纳米纤维散射而导致的延长光吸收路径引起的增强光学吸收，具有P3HT / PTB7的最佳结晶度的良好纳米形态及其与PC的良好混合 <sub> 61 </ sub> BM，以及P3HT和PTB7聚合物链的平面上的增加的面内对准，用于有效的激子解离和载流子提取，并在垂直方向上改善电荷输送。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第20期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang He Jun‐ning&option=202" target="_blank" rel="nofollow">Huang He Jun‐ning;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nan Hui Rong&option=202" target="_blank" rel="nofollow">Nan Hui Rong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Ying Guo&option=202" target="_blank" rel="nofollow">Yang Ying Guo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gao Xing Yu&option=202" target="_blank" rel="nofollow">Gao Xing Yu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Fei&option=202" target="_blank" rel="nofollow">Chen Fei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Zhi‐Kuan&option=202" target="_blank" rel="nofollow">Chen Zhi‐Kuan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrospinning&option=203" rel="nofollow">electrospinning;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanofibers&option=203" rel="nofollow">nanofibers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=organic photovoltaic&option=203" rel="nofollow">organic photovoltaic;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thick films&option=203" rel="nofollow">thick films;</a> </p> <div class="translation"> 机译：静电纺丝;纳面布勒;有机光伏;厚膜; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434946.html">Improved Performance of Thick Films Based Binary and Ternary Bulk Heterojunction Organic Photovoltaic Devices Incorporated with Electrospinning Processed Nanofibers</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang He Jun‐ning&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Huang He Jun‐ning,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nan Hui Rong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Nan Hui Rong,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Ying Guo&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yang Ying Guo,</a> <a href="/journal-foreign-18063/" target="_blank" rel="nofollow" class="tuijian_authcolor">Advanced materials interfaces .</a> <span>2018</span><span>,第20期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：基于厚膜的二元和三元散装异质结的有机光伏器件的改进性能掺入电纺丝加工纳米纤维</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704020695225.html">Bis(tri-n-alkylsilyl oxide) silicon phthalocyanines: a start to establishing a structure property relationship as both ternary additives and non-fullerene electron acceptors in bulk heterojunction organic photovoltaic devices</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dang Minh-Trung&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dang Minh-Trung,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Grant Trevor M.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Grant Trevor M.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Han&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yan Han,</a> <a href="/journal-foreign-35176/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Materials Chemistry, A. 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=郭金川&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,郭金川</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=周彬&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,周彬</a> <span> <a href="/journal-cn-56962/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 光子学报 </a> </span> <span> . 2012</span><span>,第8期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-journal-cn_chinese-journal-luminescence_thesis/0201230433516.html">辐照强度及温度对双层异质结有机光伏器件性能的影响</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李卫民&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李卫民</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=郭金川&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,郭金川</a> <a 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