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Thermoelectric properties of a quantum dot array connected to metallic electrodes

机译:连接到金属电极的量子点阵列的热电特性

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摘要

The thermoelectric properties of a quantum dot array (QDA) embedded in a nanowire connected to metallic electrodes are investigated theoretically via the extended Hubbard model in the Coulomb blockade regime. Coupled quantum dots (QDs) with dot number N = 2-5 are considered. It is found that the thermoelectric properties converge to almost the same results when N approaches 5, indicating that our results are applicable for a QDA with a large number of QDs. Our studies indicate that in order to achieve the optimal figure of merit (ZT), it is preferable to have the QD energy levels above the Fermi energy (EF) of the electrodes of the QDA junction. The effects of QD energy level and interdot coupling variations (due to the QD size and position fluctuation) on the thermoelectric properties are also examined. We find that the QD size fluctuation significantly suppresses the maximum ZT in the weak interdot hopping strength (t?,j). We also find that the Seebeck coefficient is insensitive to t?,j and the tunneling rates when the QD energy levels are far above EF. For a given t?,j and large on-site Coulomb interactions, increasing the QD number N in the QDA would suppress the maximum ZT value. It is possible to achieve an optimal ZT larger than 3 by tailoring the physical parameters of the QDA junction system.
机译:理论上,在库仑阻塞状态下,通过扩展的Hubbard模型研究了嵌入与金属电极连接的纳米线中的量子点阵列(QDA)的热电特性。考虑点号为N = 2-5的耦合量子点(QD)。发现当N接近5时,热电性能收敛到几乎相同的结果,这表明我们的结果适用于具有大量QD的QDA。我们的研究表明,为了获得最佳品质因数(ZT),最好使QD能级高于QDA结电极的费米能(EF)。还检查了QD能级和点间耦合变化(由于QD尺寸和位置波动)对热电性能的影响。我们发现,QD尺寸波动显着抑制了弱的点间跳变强度(t?,j)中的最大ZT。我们还发现,当QD能级远高于EF时,塞贝克系数对t?,j和隧穿速率不敏感。对于给定的t,j和大的库仑相互作用,增加QDA中的QD数量N将抑制最大ZT值。通过调整QDA结系统的物理参数,可以获得大于3的最佳ZT。

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