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Electromagnetic properties of a monolayer of polarisable particles deposited on graphene

机译:石墨烯上沉积的可极化颗粒单层的电磁特性

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We theoretically predict several plasmonic effects that arise when a monolayer of small polarisable particles is deposited on graphene, related to surface plasmon-polaritons (SPPs) supported by the latter in the terahertz (THz) spectral range. The electromagnetic coupling between graphene SPPs and dipole moments of the nanoparticles (NPs) gives rise to optical properties that are not present in the individual components of this system. The polarisation characteristics of the particles are modified, namely: (ⅰ) individual NP's polarisability is renormalized and (ⅱ) their dipole-dipole interaction includes, beyond the usual ∝ p~(-3) term (p is the particle-particle distance), an indirect particle-particle coupling arises via polarisation charges induced on the graphene-covered interface by each particle - this indirect coupling oscillates with the interparticle distance. We derived coupled-dipole equations taking into account all these effects, allowing us to calculate an effective optical conductivity of the particles' monolayer and study the optical properties of the composite (G+NPs) system One of the G+NPs system's unique features is a collective resonant mode, causing a considerable enhancement of the THz radiation absorption in graphene, while the reflection drops to nearly zero for a broad range of angles of incidence. The frequency of this resonant mode can be adjusted by changing the Fermi energy in graphene via electrostatic gating and therefore it can be used for electrically controlled reflection and transmission of THz radiation. Another remarkable finding is that the composite layer supports s-polarised surface polaritons linked to Drude plasmons in graphene.
机译:从理论上讲,我们预测当石墨烯上沉积一层可极化的小颗粒时所产生的几种等离激元效应,这与后者在太赫兹(THz)光谱范围内支持的表面等离激元-极化子(SPPs)有关。石墨烯SPP与纳米颗粒(NP)的偶极矩之间的电磁耦合产生了该系统各个组件中不存在的光学特性。修改了粒子的极化特性,即:(ⅰ)各个NP的极化率重新归一化;(ⅱ)它们的偶极-偶极相互作用包括超出通常的∝ p〜(-3)项(p是粒子到粒子的距离) ,通过每个粒子在石墨烯覆盖的界面上感应的极化电荷产生间接的粒子-粒子耦合-这种间接耦合随着粒子间的距离而振荡。我们考虑了所有这些影响,得出了偶合偶极子方程,使我们能够计算颗粒单层的有效光学导率,并研究复合(G + NPs)系统的光学性质。G+ NPs系统的独特之处之一是集体共振模式,大大提高了石墨烯中太赫兹辐射的吸收率,而对于大范围的入射角,反射率下降到几乎为零。可以通过通过静电门控改变石墨烯中的费米能量来调节该共振模式的频率,因此可以将其用于电控反射和传输太赫兹辐射。另一个非凡的发现是,复合层支持与石墨烯中的Drude等离子体激元相连的s极化表面极化子。

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