Provided are a photoalignment method and a photoalignment device, including: adjusting direction of light ray emitted from light source so that first angle is formed between that and XOY plane, and second angle is formed between projection of that on XOY plane and Y-axis; adjusting angle of polarizing plate so that it is parallel to XOY plane, and its light transmission axis is parallel to projection of that on XOY plane; moving array substrate along negative direction of Y-axis to perform exposure operation on array substrate; and moving color filter substrate, which rotated by 180 degrees, in negative direction of Y-axis to perform exposure operation on color filter substrate, wherein color filter substrate has exposure regions which are completely identical, in position and number, to those of array substrate, and each exposure region is exposed to light in identical direction to that of corresponding exposure region of array substrate.
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