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Coupled plasmon-exciton induced transparency and slow light in plexcitonic metamaterials

机译:耦合等离子体激元激子诱导透明度和plexcitonic超材料中的慢光

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摘要

Classical analogues of the well-known effect of electromagnetically induced transparency (EIT) in quantum optics have been the subject of considerable research in recent years from microwave to optical frequencies, because of their potential applications in slow light devices, studying nonlinear effects in low-loss nanostructures, and development of low-loss metamaterials. A large variety of plasmonic structures has been proposed for producingclassical EIT-like effects in different spectral ranges. The current approach for producing plasmon-induced transparency is usually based on precise design of plasmonic “molecules,” which can provide specific interacting dark and bright plasmonic modes with Fano-type resonance couplings. In this paper, we show that classical interactions of coupled plasmonic and excitonic spherical nanoparticles (NPs) can result in much more effective transparency and slow light effects in metamaterials composed of such coupled NPs. To reveal more details of the wave-particle and particle-particle interactions, the electric field distribution and field lines of Poynting vector inside and around the NPs are calculated using the finite element method. Finally, using extended MaxwellGarnett theory, we study the coupled-NP-induced transparency and slow light effects in a metamaterial comprising random mixture of silver and copper chloride (CuCl) NPs, and more effectively in a metamaterial consisting of random distribution of coated NPs with CuCl cores and aluminum shells in the UV region.
机译:近年来,从微波到光频率的量子光学中众所周知的电磁感应透明(EIT)效应的经典类似物,由于其在慢光设备中的潜在应用,正在研究低辐射的非线性效应,因此受到了广泛的研究。损耗纳米结构,以及低损耗超材料的发展。已经提出了各种各样的等离子体结构,以在不同的光谱范围内产生经典的EIT样效应。当前产生等离激元引起的透明性的方法通常是基于等离激元“分子”的精确设计,它可以提供具有Fano型共振耦合的特定相互作用的暗和亮等离激元模式。在本文中,我们表明,等离激元和激子球形纳米粒子(NP)的经典相互作用可以在由此类耦合NP组成的超材料中产生更有效的透明性和减慢光的影响。为了揭示波粒和粒子之间相互作用的更多细节,使用有限元方法计算了NP内部和周围的Poynting向量的电场分布和场线。最后,使用扩展的MaxwellGarnett理论,我们在包含银和氯化铜(CuCl)NP随机混合物的超材料中研究了耦合NP诱导的透明性和慢光效应,更有效地研究了由包覆NP随机分布的超材料组成的超材料UV区域中的CuCl芯和铝壳。

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