Wepresent the first measurement of the vectorial response of strongly dressed helium atoms probed by an attosecond pulse train (APT) polarised either parallel or perpendicular to the dressing field polarisation. The transient absorption is probed as a function of delay between the APT and the Linearly polarised 800 nmfield of peak intensity 1.3∗1014 W cm-2. The APT spans the photon energy range 1642 eV, covering the first ionisation energy of helium (24.59 eV). With parallel polarised dressing and probing fields, we observe modulations with periods of one half and one quarter of the dressing field period. When the polarisation of the dressing field is altered from parallel to perpendicular with respect to the APT polarisation we observe a large suppression in the Modulation depth of the above ionisation threshold absorption. In addition to this we present the intensity dependence of the harmonic modulation depth as a function of delay between the dressing and probe fields, with dressing field peak intensities ranging from 2∗1012 to 2∗1014 W cm-2.We compare our experimental results with a full-dimensional solution of the single-atom time-dependent (TD) Schrdinger equation obtained using the recently developed abinitio TDB-spline ADCmethod and find good qualitative agreement for the above threshold harmonics.
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机译:我们介绍了由被平行或垂直于修整场极化极化的阿秒脉冲串(APT)探测到的强打扮氦原子矢量响应的首次测量。根据APT和峰值强度为1.3 * 1014 W cm-2的线性偏振800 nm场之间的延迟来探测瞬态吸收。 APT跨越光子能量范围1642 eV,涵盖了氦的第一电离能(24.59 eV)。对于平行极化的修整场和探测场,我们观察到的调制周期为修整场周期的一半和四分之一。当修整场的极化相对于APT极化从平行更改为垂直时,我们观察到上述电离阈值吸收的调制深度受到很大抑制。除此之外,我们提出了谐波调制深度的强度依赖性,它是修整场和探测场之间延迟的函数,修整场的峰值强度范围为2 * 1012至2 * 1014 W cm-2。我们比较了实验结果使用最近开发的二叉树TDB样条ADC方法获得的单原子时变(TD)Schrdinger方程的全尺寸解,并为上述阈值谐波找到了良好的定性一致性。
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