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Magnetic ordering and transport properties of PrBa2Cu4O8

机译:PrBa2Cu4O8的磁有序和输运性质

摘要

[[abstract]]We present studies of the thermal, magnetic, and electrical transport properties of polycrystalline PrBa2Cu4O8 prepared at ambient oxygen pressure. Measurements of the low temperature specific heat C(T) and magnetic susceptibility X(T) show similar results as in PrBa2Cu4O8 an anomaly observed at 17 K in C(T) and dχ/dT may be due to the antiferromagnetic ordering of the Pr sublattice. The upper limit of the entropy associated with the magnetic ordering is estimated to be 6.6 J/mol K. The free magnetic moment from a simple Curie-Weiss fit is 3.11 μg. These similarities in magnetic properties of PrBa2Cu3O7 and PrBa2Cu4O8 suggest that the magnetic coupling mechanism might be mainly associated with the CuO2, planes. The resistivity p(T) is nearly metallic from 1.5 to 300 K. Comparisons of samples prepared by different methods suggest that the anomaly in resistivity around 200 K may be extrinsic. The behavior of p(T) is rather puzzling and cannot be explained simply by a dimensional crossover of charge transport arising from the double CuO2 chains. Other similarities and differences of the mentioned physical properties between PrBa2Cu4O8 and PrBa2Cu4O8 are stressed as well
机译:[[摘要]]我们研究在环境氧气压力下制备的多晶PrBa2Cu4O8的热,磁和电传输性质。低温比热C(T)和磁化率X(T)的测量显示出与PrBa2Cu4O8类似的结果,在C(T)和dχ/ dT中于17 K观察到的异常可能是由于Pr亚晶格的反铁磁有序。与磁有序相关的熵的上限估计为6.6 J / molK。来自简单居里-魏斯拟合的自由磁矩为3.11μg。 PrBa2Cu3O7和PrBa2Cu4O8在磁性方面的这些相似性表明,磁耦合机理可能主要与CuO2平面有关。电阻率p(T)在1.5到300 K之间几乎是金属。通过不同方法制备的样品的比较表明,在200 K附近的电阻率异常可能是外在的。 p(T)的行为令人费解,无法简单地解释由双CuO2链引起的电荷传输的尺寸交叉。还强调了PrBa2Cu4O8和PrBa2Cu4O8之间提到的物理性能的其他相似性和差异

著录项

  • 作者

    Yang H.D.;

  • 作者单位
  • 年度 2011
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  • 原文格式 PDF
  • 正文语种 [[iso]]en
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