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Quantitative TEM imaging of the magnetostructural and phase transitions in FeRh thin film systems

机译:FeRh薄膜系统中磁畴结构和相变的定量TEm成像

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摘要

Equi-atomic FeRh is a very interesting material as it undergoes a magnetostructural transition from an antiferromagnetic (AF) to a ferromagnetic (FM) phase between 75-105 °C. Its ability to present phase co-existence separated by domain walls (DWs) above room temperature provides immense potential for exploitation of their DW motion in spintronic devices. To be able to effectively control the DWs associated with AF/FM coexistence in FeRh thin films we must fully understand the magnetostructural transition and thermomagnetic behaviour of DWs at a localised scale. Here we present a transmission electron microscopy investigation of the transition in planar FeRh thin-film samples by combining differential phase contrast (DPC) magnetic imaging with in situ heating. We perform quantitative measurements from individual DWs as a function of temperature, showing that FeRh on NiAl exhibits thermomagnetic behaviour consistent with the transition from AF to FM. DPC imaging of an FeRh sample with HF-etched substrate reveals a state of AF/FM co-existence and shows the transition from AF to FM regions proceeds via nucleation of small vortex structures, which then grow by combining with newly nucleated vortex states into larger complex magnetic domains, until it is in a fully-FM state.
机译:等原子FeRh是一种非常有趣的材料,因为它会在75-105°C之间经历从反铁磁(AF)到铁磁(FM)相的磁结构转变。它具有呈现在室温以上被畴壁(DW)隔开的相位共存的能力,为在自旋电子设备中利用其DW运动提供了巨大的潜力。为了能够有效控制与FeRh薄膜中AF / FM共存相关的DW,我们必须在局部范围内充分了解DW的磁结构转变和热磁行为。在这里,我们通过结合差分相衬对比度(DPC)磁成像技术和原位加热技术,对平面FeRh薄膜样品中的转变进行了透射电子显微镜研究。我们对各个DW随温度进行定量测量,结果表明NiAl上的FeRh表现出与从AF到FM转变一致的热磁行为。 FeRh样品经HF蚀刻后的基质的DPC成像揭示了AF / FM共存的状态,并显示了从AF到FM区域的转变是通过小涡旋结构的成核而进行的,然后通过与新成核的涡旋状态结合成更大的直到处于完全FM状态为止。

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