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Theoretical characterization of the collective resonance states underlying the xenon giant dipole resonance

机译:氙巨偶极共振背后集体共振态的理论刻画

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摘要

We present a detailed theoretical characterization of the two fundamental collective resonances underlying the xenon giant dipole resonance (GDR). This is achieved consistently by two complementary methods implemented within the framework of the configuration-interaction singles (CIS) theory. The first method accesses the resonance states by diagonalizing the many-electron Hamiltonian using the smooth exterior complex scaling technique. The second method involves a different application of the Gabor analysis to wave-packet dynamics. We identify one resonance at an excitation energy of 74 eV with a lifetime of 27 as and the second at 107 eV with a lifetime of 11 as. Our work provides a deeper understanding of the nature of the resonances associated with the GDR: a group of close-lying intrachannel resonances splits into two far-separated resonances through interchannel couplings involving the 4d electrons. The CIS approach allows a transparent interpretation of the two resonances as new collective modes. Due to the strong entanglement between the excited electron and the ionic core, the resonance wave functions are not dominated by any single particle-hole state. This gives rise to plasma-like collective oscillations of the 4d shell as a whole.
机译:我们介绍了氙巨偶极子共振(GDR)背后的两个基本集体共振的详细理论特征。这是通过在配置相互作用单(CIS)理论框架内实施的两种互补方法一致地实现的。第一种方法是使用光滑外部复比例缩放技术通过对角多电子哈密顿量来访问共振状态。第二种方法涉及将Gabor分析应用于波包动力学。我们确定了一个激发能量为74 eV,寿命为27 as的共振,第二个共振为107 eV,寿命为11 as的共振。我们的工作使人们对与GDR相关的共振的性质有了更深的理解:一组紧密的通道内共振通过涉及4d电子的通道间耦合分裂为两个相距很远的共振。 CIS方法允许将两个共振透明地解释为新的集体模式。由于受激电子与离子核之间的强力缠结,共振波函数不受任何单个粒子-空穴状态的支配。整体上,这会引起4d外壳的类似等离子体的集体振荡。

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