Structure-properties relationships in solution-processable single-material molecular emitters for efficient green organic light-emitting diodes

摘要

The electroluminescent properties of a series of solution-processable fluorescent molecular emitters have been systematically investigated. While the introduction of the electron-deficient benzothiadiazole unit in the structure confers efficient electron-injection on the emitter materials, they exhibit different hole-transport properties. The device characteristics of the OLEDs based on these various emitters are discussed on the basis of (i) the energy levels of their HOMO and LUMO and (ii) their hole-transport properties in relation with the charge-transport and blocking properties of the electron- and hole-transport layers. (C) 2012 Elsevier B.V. All rights reserved.