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Resonant excitation of confined excitons in nanocrystal quantum dots using surface plasmon-polaritons

机译:利用表面等离振子-极化子共振激发纳米晶体量子点中的受激激子

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摘要

Surface plasmon-polaritons (SPPs) in a multilayerstructure consisting of a metallic film and one or more layers ofnanocrystal (NC) quantum dots (QDs) are studied theoretically. Itis shown that there is a resonance coupling between the plasmonpolaritonspropagating along the metal/NC-layer interface andexcitons confined in the dots, which produces a considerable effecton the optical properties of the structure unless the dispersion ofthe QD size is too large. Using a transfer matrix formalism,multilayer structures consisting of NC composite and metallic films are considered and it is demonstrated that the couplingextends over several layers constituting the structure. It can be explored in order to selectively excite QDs of different size bymaking a layer-by layer assembled NC planar structure and using an attenuated total reflection (ATR) configuration for the SPPenhancedexcitation of the dots. In particular, it opens the possibility to control the relative intensity of light of different color,emitted by the QDs of different size.
机译:理论上研究了由金属膜和一层或多层纳米晶体(NC)量子点(QDs)组成的多层结构中的表面等离振子-极化子(SPPs)。结果表明,沿着金属/ NC层界面传播的等离激元极化子与局限在点中的激子之间存在共振耦合,除非QD尺寸的色散太大,否则这会对结构的光学性能产生相当大的影响。使用传递矩阵形式,考虑了由NC复合材料和金属膜组成的多层结构,并证明了耦合扩展到构成结构的几层上。可以进行探索,以便通过制作逐层组装的NC平面结构并将衰减全反射(ATR)配置用于点的SPP增强来有选择地激发不同尺寸的QD。特别地,这为控制由不同尺寸的量子点发出的不同颜色的光的相对强度提供了可能性。

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