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What causes the irregular cycle of the atmospheric tape recorder signal in HCN?

机译:是什么原因导致HCN中的大气磁带录音机信号出现不规则的循环?

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摘要

Variations in the mixing ratio of long-lived trace gases entering the stratosphere in the tropics are carried upward with the rising air with the signal being observable throughout the tropical lower stratosphere. This phenomenon, referred to as "atmospheric tape recorder" has previously been observed for water vapor, CO2, and CO which exhibit an annual cycle. Recently, based on Microwave Limb Sounder (MLS) and the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) satellite measurements, the tape recorder signal has been observed for hydrogen cyanide (HCN) but with an approximately two-year period. Here we report on a model simulation of the HCN tape recorder for the time period 2002-2008 using the Chemical Lagrangian Model of the Stratosphere (CLaMS). The model can reproduce the observed pattern of the HCN tape recorder signal if time-resolved emissions from fires in Indonesia are used as lower boundary condition. This finding indicates that inter-annual variations in biomass burning in Indonesia, which are strongly influenced by El Nino events, control the HCN tape recorder signal. A longer time series of tropical HCN data will probably exhibit an irregular cycle rather than a regular biannual cycle. Citation: Pommrich, R., R. Muller, J.-U. Grooss, G. Gunther, P. Konopka, M. Riese, A. Heil, M. Schultz, H.-C. Pumphrey, and K. A. Walker (2010), What causes the irregular cycle of the atmospheric tape recorder signal in HCN?, Geophys. Res. Lett., 37, L16805, doi:10.1029/2010GL044056.
机译:进入热带平流层的长寿命微量气体混合比的变化随着空气的上升而向上传播,整个热带低平流层都可以观测到该信号。以前已经观察到这种现象,称为“大气带记录仪”,这种现象表现为水蒸汽,二氧化碳和一氧化碳的年循环。近来,基于微波无声测深仪(MLS)和大气化学实验傅立叶变换光谱仪(ACE-FTS)卫星测量,已经观察到磁带记录仪信号中的氰化氢(HCN),但周期约为两年。在这里,我们使用平流层化学拉格朗日模型(CLaMS)报告了2002-2008年期间HCN录音机的模型仿真。如果将印度尼西亚大火的时间分辨排放量用作下边界条件,则该模型可以重现HCN磁带记录器信号的观察模式。这一发现表明,受厄尔尼诺事件的强烈影响,印度尼西亚生物质燃烧的年际变化控制着HCN录音机信号。较长时间的热带HCN数据序列可能会显示出不规则的周期,而不是规则的半年周期。引用:Pommrich,R.,R. Muller,J.-U。 Grooss,G。Gunther,P。Konopka,M。Riese,A。Heil,M。Schultz,H.-C。 Pumphrey和K. A. Walker(2010),什么原因导致HCN中的大气磁带录音机信号出现不规则循环?Geophys。 Res。 Lett。,37,L16805,doi:10.1029 / 2010GL044056。

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