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Dichroic coherent diffractive imaging

机译:二向色相干衍射成像

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摘要

Understanding electronic structure at the nanoscale is crucial to untangling fundamental physics puzzles such as phase separation and emergent behavior in complex magnetic oxides. Probes with the ability to see beyond surfaces on nanometer length and subpicosecond time scales can greatly enhance our understanding of these systems and will undoubtedly impact development of future information technologies. Polarized X-rays are an appealing choice of probe due to their penetrating power, elemental and magnetic specificity, and high spatial resolution. The resolution of traditional X-ray microscopes is limited by the nanometer precision required to fabricate X-ray optics. Here we present a novel approach to lensless imaging of an extended magnetic nanostructure, in which a scanned series of dichroic coherent diffraction patterns is recorded and numerically inverted to map its magnetic domain configuration. Unlike holographic methods, it does not require a reference wave or precision optics. In addition, it enables the imaging of samples with arbitrarily large spatial dimensions, at a spatial resolution limited solely by the coherent X-ray flux, wavelength, and stability of the sample with respect to the beam. It can readily be extended to nonmagnetic systems that exhibit circular or linear dichroism. We demonstrate this approach by imaging ferrimagnetic labyrinthine domains in a Gd/Fe multilayer with perpendicular anisotropy and follow the evolution of the domain structure through part of its magnetization hysteresis loop. This approach is scalable to imaging with diffraction-limited resolution, a prospect rapidly becoming a reality in view of the new generation of phenomenally brilliant X-ray sources.
机译:了解纳米级的电子结构对于解决基本的物理难题(例如相分离和复杂磁性氧化物中的出射行为)至关重要。能够在纳米级和亚皮秒级的尺度上超越表面的探头可以极大地增强我们对这些系统的理解,并且无疑会影响未来信息技术的发展。极化X射线具有穿透力,元素和磁性特异性以及高空间分辨率等优点,因此成为探针的诱人选择。传统X射线显微镜的分辨率受到制造X射线光学器件所需的纳米精度的限制。在这里,我们提出了一种扩展的磁性纳米结构的无透镜成像的新颖方法,其中记录了一系列扫描的二向色相干衍射图案,并对其进行了数值反转以映射其磁畴配置。与全息方法不同,它不需要参考波或精密光学器件。另外,它使得能够以仅由相干X射线通量,波长和样品相对于光束的稳定性限制的空间分辨率来成像具有任意大的空间尺寸的样品。它可以很容易地扩展到表现出圆形或线性二向色性的非磁性系统。我们通过在具有垂直各向异性的Gd / Fe多层膜中成像亚铁磁迷宫结构域并通过其磁化磁滞回线跟踪结构域结构的演变来证明这种方法。这种方法可扩展到具有衍射极限分辨率的成像,鉴于新一代异常出色的X射线源,这种前景迅速成为现实。

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