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Exactly Solvable Light-Matter Interaction Models for Studying Filamentation Dynamics

机译:研究细丝动力学的完全可解决的轻质相互作用模型

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摘要

This dissertation demonstrates the usefulness of exactly solvable quantum models in the investigation of light-matter interaction phenomena associated with the propagation of ultrashort laser pulses through gaseous media. This work fits into the larger research effort towards remedying the weaker portions of the standard set of medium modeling equations commonly used in simulations. The ultimate goal is to provide a self-consistent quantum mechanical description that can integrate Maxwell and Schrödinger systems and provide a means to realistically simulate nonlinear optical experiments on relevant scales. The study of exactly solvable models begins with one of the simplest quantum systems available, one with a 1D Dirac-delta function potential plus interaction with the light field. This model contains, in the simplest form, the most important "ingredients" that control optical filamentation, i.e. discrete and continuum electronic states. The importance of both states is emphasized in the optical intensity regime in which filaments form, where both kinds of electronic states simultaneously play a role and may not even be distinguishable. For this model atom, an analytical solution for the time-dependent light-induced atomic response from an arbitrary excitation waveform is obtained. Although this system is well-known and has been studied for decades, this result is probably the most practically useful and general one obtained thus far. Numerical implementation details of the result are also given as the task is far from trivial. Given an efficient implementation, the model is used in light-matter interaction simulations and from these it is apparent that even this toy model can qualitatively reproduce many of the nonlinear phenomena seen in experiments. Not only does this model capture the basic physics of optical filamentation, but it is also well-suited for high harmonic generation simulations. Next, a theoretical framework for using Stark resonant states (or metastable states) to represent the medium's polarization response is presented. Researchers have recognized long ago the utility of Gamow resonant states as a description of various decay processes. Even though a bound electron experiences a similar decay-like process as it transitions into the continuum upon ionization, it was unclear whether field-induced Stark resonant states carry physically relevant information. It is found that they do, and in particular it is possible to use them to capture a medium's polarization response. To this end, two quantum systems with potentials represented by a 1D Dirac-delta function and a 1D square well are solved, and all the necessary quantities for their use as medium models are presented. From these results it is possible to conjecture some general properties that hold for all resonance systems, including systems that reside in higher than one dimensional space. Finally, as a practical application of this theory, the Metastable Electronic State Approach (MESA) is presented as a quantum-based replacement for the standard medium modeling equations.
机译:这篇论文证明了精确可解的量子模型在研究与超短激光脉冲通过气体介质传播有关的光-物质相互作用现象中的有用性。这项工作适合进行较大的研究工作,以弥补模拟中常用的标准介质建模方程组的较弱部分。最终目的是提供一个自洽的量子力学描述,该描述可以集成麦克斯韦系统和薛定er系统,并提供一种在相关规模上真实地模拟非线性光学实验的方法。对精确可解模型的研究始于现有的最简单的量子系统之一,其中一个具有一维狄拉克-德尔塔函数势以及与光场的相互作用。该模型以最简单的形式包含控制光丝的最重要的“成分”,即离散和连续电子态。这两种状态的重要性在形成灯丝的光学强度体系中得到了强调,其中两种电子状态同时发挥作用,甚至可能无法区分。对于此模型原子,从任意激发波形中获得了随时间变化的光诱导原子响应的解析解。尽管该系统是众所周知的,并且已经研究了数十年,但是该结果可能是迄今为止获得的最实用和最通用的结果。还给出了结果的数字实现细节,因为任务远非轻而易举。给定有效的实现方式,该模型可用于光-物质相互作用模拟中,并且由此可见,即使是这种玩具模型也可以定性地再现实验中看到的许多非线性现象。该模型不仅捕获了光学纤维的基本物理原理,而且非常适合于高谐波生成模拟。接下来,提出了使用斯塔克共振态(或亚稳态)表示介质极化响应的理论框架。研究人员早已认识到Gamow共振态作为各种衰变过程的描述的用途。尽管束缚电子在电离时过渡到连续体时会经历类似的衰变状过程,但尚不清楚场感应的Stark共振态是否携带物理上相关的信息。发现它们确实存在,特别是可以使用它们捕获介质的极化响应。为此,解决了两个具有一维狄拉克-德尔塔函数和一维方阱的势能的量子系统,并提出了用作其介质模型的所有必要量。根据这些结果,可以推测出对于所有共振系统都适用的一些一般属性,包括驻留在一维以上空间中的系统。最后,作为该理论的实际应用,提出了亚稳态电子状态方法(MESA),作为基于量子的标准介质建模方程式替代。

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    Brown Jeffrey Michael;

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  • 年度 2016
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  • 原文格式 PDF
  • 正文语种 en_US
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