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Size-dependent effect of gold nanospheres on the acoustic pressure pulses from laser-irradiated suspensions

机译:金纳米球对激光辐照悬浮液声压脉冲的尺寸依赖性效应

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摘要

We carried out the experimental measurements of photoacoustic responses, where the suspensions of spherical gold nanoparticles (NPs) of different diameters (20, 40, and 50 nm) in water at different concentrations and different temperatures (4 and 20 °C) were irradiated by 0.8-ns laser pulses. In the case of 20 °C, the values of photoacoustic signals normalized by the light absorbance of the NP suspension decreased with increasing the NP size. The photoacoustic signals at 4 °C were significantly reduced compared with those at 20 °C. These experimental results are in fair agreement with the estimations from our phenomenological model, where the acoustic pressure pulse is represented by a sum of two contributions from the NPs and the surrounding liquid medium.
机译:我们进行了光声响应的实验测量,其中分别用不同的浓度和温度(4和20°C)照射直径不同(20、40和50 nm)的球形金纳米颗粒(NP)在水中的悬浮液0.8 ns的激光脉冲。在20°C的情况下,通过NP悬浮液的吸光度归一化的光声信号值随NP尺寸的增加而降低。与20°C相比,在4°C下的光声信号显着降低。这些实验结果与我们的现象学模型的估计非常吻合,在该模型中,声压脉冲由NP和周围液体介质的两个贡献之和表示。

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