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Thickness Dependent Magnetic Anisotropy of Ultrathin LCMO Epitaxial Thin Films

机译:超薄LCMO外延薄膜的厚度依赖性磁各向异性

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摘要

The magnetic properties of La_0.7Ca_0.3Mn_O3 (LCMO) manganite thin films were studied with magnetometry and ferromagnetic resonance as a function of film thickness. They maintain the colossal magnetoresistance behavior with a pronounced metal-insulator transition around 150-200 K, except for the very thinnest films studied (3 nm). Nevertheless, LCMO films as thin as 3 nm remain ferromagnetic, without a decrease in saturation magnetization, indicating an absence of dead-layers, although below approximately 6 nm the films remain insulating at low temperature. Magnetization hysteresis loops reveal that the magnetic easy axes lie in the plane of the film for thicknesses in the range of 4-15 nm. Ferromagnetic resonance studies confirm that the easy axes are in-plane, and find a biaxial symmetry in-plane with two, perpendicular easy axes. The directions of the easy axes with respect to the crystallographic directions of the cubic SrTiO_3 substrate differ by 45 deg in 4- and 15-nm-thick LCMO films.
机译:研究了La_0.7Ca_0.3Mn_O3(LCMO)锰矿薄膜的磁性能,其磁学和铁磁谐振与薄膜厚度有关。它们保持了巨大的磁阻性能,并且在大约150-200 K的范围内具有明显的金属-绝缘体转变,但研究的最薄薄膜(3 nm)除外。尽管如此,薄至3 nm的LCMO膜仍保持铁磁性,而饱和磁化强度却没有降低,这表明没有死层,尽管在大约6 nm以下,该膜仍在低温下保持绝缘。磁化磁滞回线表明,磁易轴位于薄膜平面内,厚度范围为4-15 nm。铁磁共振研究证实了易轴在平面内,并找到了具有两个垂直易轴的双轴对称面。相对于立方SrTiO_3衬底的晶体学方向,易轴方向在4纳米和15纳米LCMO薄膜中相差45度。

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