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Biexciton and Triexciton States in Quantum Dots in the Weak Confinement Regime

机译:弱约束条件下量子点中的双激子态和三激子态

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摘要

Biexciton and triexciton states in CuCl quantum dots were studied by means of time-resolved size-selective pump-and-probe technique. A clear induced absorption band is observed on the high-energy side of the excitation photon energy. The new induced absorption is assigned to the transition from the exciton ground state to one of the weakly correlated exciton pair states which were theoretically predicted to exist and to play an important role in nonlinear optical processes. Its pump energy dependence and temporal evolution strongly support this assignment. Under high-density or two-color excitation condition, a triexciton state in quantum dots is observed for the first time.
机译:利用时间分辨尺寸选择泵浦和探针技术研究了CuCl量子点中的双激子和三激子态。在激发光子能量的高能侧观察到清晰的感应吸收带。新的诱导吸收被指定为从激子基态到弱相关激子对状态之一的过渡,这在理论上被预测为存在并在非线性光学过程中起重要作用。其泵浦能量依赖性和时间演变强烈支持这一任务。在高密度或双色激发条件下,首次观察到量子点中的三激子态。

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