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Thermal and fast neutron detection in chemical vapor deposition single-crystal diamond detectors

机译:化学气相沉积单晶金刚石探测器中的热中子探测和快速中子探测

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摘要

Recently, a compact solid-state neutron detector capable of simultaneously detecting thermal and fast neutrons was proposed [M. Marinelli et al., Appl. Phys. Lett. 89, 143509 (2006)]. Its design is based on a p-type/intrinsic/metal layered structure obtained by Microwave Plasma Chemical Vapor Deposition (CVD) of homoepitaxial diamond followed by thermal evaporation of an Al contact and a LiF converting layer. Fast neutrons are directly detected in the CVD diamond bulk, since they have enough energy to produce the C(n, α)Be reaction in diamond. Thermal neutrons are instead converted into charged particles in the LiF layer through the Li(n, α)T nuclear reaction. These charged particles are then detected in the diamond layer. The thickness of the LiF converting layer and the CVD diamond sensing layer affect the counting efficiency and energy resolution of the detector both for low- (thermal) and high-energy neutrons. An analysis is carried out on the dynamics of the Li(n, α)T and the C(n, α)Be reactions products, and the distribution of the energy released inside the sensitive layer is calculated. The detector counting efficiency and energy resolution were accordingly derived as a function of the thickness of the LiF and CVD diamond layers, both for thermal and fast neutrons, thus allowing us to choose the optimum detector design for any particular application. Comparison with experimental results is also reported.
机译:近来,提出了一种能够同时检测热中子和快中子的紧凑型固态中子探测器[M. Marinelli等,Appl.Chem.Soc。物理来吧89,143509(2006)]。其设计基于通过同质外延金刚石的微波等离子体化学气相沉积(CVD),然后热蒸发Al接触层和LiF转换层获得的p型/本征/金属层状结构。快速中子可以直接在CVD金刚石块中检测到,因为它们具有足够的能量来在金刚石中产生C(n,α)Be反应。相反,热中子通过Li(n,α)T核反应在LiF层中转换为带电粒子。然后,在金刚石层中检测到这些带电粒子。 LiF转换层和CVD金刚石感应层的厚度会影响低(热)中子和高能中子的计数效率和探测器的能量分辨率。对Li(n,α)T和C(n,α)Be反应产物的动力学进行了分析,并计算了敏感层内部释放的能量分布。因此,对于热中子和快中子,探测器的计数效率和能量分辨率是LiF和CVD金刚石层厚度的函数,因此,我们可以为任何特定应用选择最佳的探测器设计。还报道了与实验结果的比较。

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