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Design and Synthesis of Enantiopure Tetrakis(pentafluorophenyl) Borate Analogues for Asymmetric Counteranion Directed Catalysis

机译：对映异常（五氟苯基）硼酸盐的设计与合成不对称抗衡催化催化

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摘要

The design and five-step synthesis of chiral tetrakis(pentafluorophenyl) borate analogues from commercially available enantiopure BINOL is described. The chiral anions have been tested in a catalytic asymmetric Mukaiyama aldol reaction.

机译：描述了来自市售的闭合Binol的手性四胞胎（五氟苯基）硼酸盐类似物的设计和五步合成。手性阴离子已在催化不对称Mukaiyama Aldol反应中进行测试。

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Benjamin List; Chandra De; Raja Mitra;
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年度 2017
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1. Design and Synthesis of Enantiopure Tetrakis(pentafluorophenyl) Borate Analogues for Asymmetric Counteranion Directed Catalysis [J] . De Chandra Kanta, Mitra Raja, List Benjamin Synlett . 2017,第18期

机译：对映异常（五氟苯基）硼酸盐的设计与合成不对称抗衡催化催化
2. Synthesis and characterization of acetonitrile-ligated transition-metal complexes with tetrakis(pentafluorophenyl)borate as counteranions [J] . Hijazi AK, Al Hmaideen A, Syukri S, European journal of inorganic chemistry . 2008,第18期

机译：以四（五氟苯基）硼酸酯为抗衡阴离子的乙腈连接的过渡金属配合物的合成与表征
3. Design and synthesis of enantiopure 1-[1(S)-(2-pyridyl)alkyl]-2(R)-isopropylaziridines, new ligands for asymmetric catalysis [J] . Katia Fiore, Gianluca Martelli, Magda Monari, Tetrahedron, Asymmetry: The International Journal for Repid Publication on all Aspects of Asymmetry in Orgainc, Inorganic, Organometallic, Physical and Bio-Organic Chemistry . 1999,第24期

机译：对映纯1- [1（S）-（2-吡啶基）烷基] -2（R）-异丙基氮丙啶的设计与合成，用于不对称催化的新配体
4. A Powerful Chiral Counteranion Motif for Asymmetric Catalysis [C] . Constantinos Rabalakos, Pilar Garcia-Garcia, Frank Lay European Symposium on Organic Chemistry . 2009

机译：一种强大的手性对抗主题用于不对称催化
5. Part I. Asymmetric organocatalysis: (1) Direct enantioselective organocatalytic hydroxymethylation of aldehydes catalyzed by alpha,alpha-diphenylprolinol trimethylsilyl ether: Application in the formal synthesis of (-)-Rasfonin; (2) Synthesis of a novel bicyclic secondary amine organocatalyst: Application to the direct enantioselective organocatalytic hydroxymethylation of aldehydes. Part II. Asymmetric synthesis of bicyclic analogues of the anti-osteoporotic drug risedronate. [D] . Miller, John Robert. 2010

机译：第一部分，不对称有机催化：（1）α，α-二苯基脯氨醇三甲基甲硅烷基醚催化的醛的直接对映选择性有机催化羟甲基化：在（-）-Rasfonin的正式合成中的应用；（2）新型双环仲胺有机催化剂的合成：应用于醛的直接对映选择性有机催化羟甲基化。第二部分抗骨质疏松药物Risedronate的双环类似物的不对称合成。
6. Asymmetric counteranion-directed Lewis acid organocatalysis for the scalable cyanosilylation of aldehydes [O] . Zhipeng Zhang, Han Yong Bae, Joyram Guin, -1

机译：不对称抗衡阴离子导向的路易斯酸有机催化醛的可扩展氰基硅烷化
7. A Structurally Robust Chiral Borate Ion: Molecular Design, Synthesis, and Asymmetric Catalysis [O] . Daisuke Uraguchi, Fumito Ueoka, Naoya Tanaka, 2020

机译：结构鲁棒的手性硼酸硼离子：分子设计，合成和不对称催化
8. Synthesis and X-ray Crystal Structures of (Au(CH2)2PPh2)2(CF3)2, (Au(CH2)2PPh2)2(C6F5)2, and (PPN)(Au(C6F5)4): Two Dinuclear Gold (II) Ylide Complexes Containing Alkyl and Aryl Ligands and a Tetrakis(pentafluorophenyl)aurate(III) [R] . Murray, H. H., Fackler, J. P., Porter, L. C., 1987

机译：（au（CH2）2pph2）2（CF3）2，（au（CH2）2pph2）2（C6F5）2和（ppN）（au（C6F5）4）的合成和X射线晶体结构：两个双核金（ II）含有烷基和芳基配体的Ylide配合物和四（五氟苯基）丙酸酯（III）

Design and Synthesis of Enantiopure Tetrakis(pentafluorophenyl) Borate Analogues for Asymmetric Counteranion Directed Catalysis

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