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The impact of bark beetle infestations on monoterpene emissions and secondary organic aerosol formation in western North America

机译:北美西部树皮甲虫侵染对单萜排放和次生有机气溶胶形成的影响

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摘要

Over the last decade, extensive beetle outbreaks in western North Americahave destroyed over 100 000 km of forest throughout British Columbiaand the western United States. Beetle infestations impact monoterpeneemissions through both decreased emissions as trees are killed (mortalityeffect) and increased emissions in trees under attack (attack effect). Weuse 14 yr of beetle-induced tree mortality data together with beetle-inducedmonoterpene emission data in the National Center for Atmospheric Research(NCAR) Community Earth System Model (CESM) to investigate the impact ofbeetle-induced tree mortality and attack on monoterpene emissions andsecondary organic aerosol (SOA) formation in western North America.Regionally, beetle infestations may have a significant impact on monoterpeneemissions and SOA concentrations, with up to a 4-fold increase inmonoterpene emissions and up to a 40% increase in SOA concentrations insome years (in a scenario where the attack effect is based on observedlodgepole pine response). Responses to beetle attack depend on the extent ofprevious mortality and the number of trees under attack in a given year,which can vary greatly over space and time. Simulated enhancements peak in2004 (British Columbia) and 2008 (US). Responses to beetle attack are shownto be substantially larger (up to a 3-fold localized increase in summertimeSOA concentrations) in a scenario based on bark-beetle attack in sprucetrees. Placed in the context of observations from the IMPROVE network, thechanges in SOA concentrations due to beetle attack are in most cases smallcompared to the large annual and interannual variability in total organicaerosol which is driven by wildfire activity in western North America. Thisindicates that most beetle-induced SOA changes are not likely detectable incurrent observation networks; however, these changes may impede efforts toachieve natural visibility conditions in the national parks and wildernessareas of the western United States.
机译:在过去的十年中,北美西部广泛的甲虫暴发已经摧毁了不列颠哥伦比亚省和美国西部超过10万公里的森林。甲虫的侵染通过杀死树木减少排放(致命效应)和受到攻击的树木增加排放(攻击效应),从而影响单萜类植物的排放。我们在国家大气研究中心(NCAR)社区地球系统模型(CESM)中使用了14年的甲虫诱发的树木死亡率数据以及甲虫诱发的单萜排放数据,以调查甲虫引起的树木死亡率和攻击对单萜排放和次生有机物的影响北美西部地区的气溶胶(SOA)形成。甲虫侵染可能对单萜和SOA浓度产生重大影响,在某些年份中,单萜的排放量最多增加4倍,SOA浓度最多增加40%(在攻击效果是基于观察到的红松反应的场景)。对甲虫袭击的反应取决于过去一年的死亡率和在特定年份被袭击的树木数量,这些随时间和空间变化很大。模拟增强在2004年(不列颠哥伦比亚省)和2008年(美国)达到峰值。在基于云杉的树皮-甲虫袭击的情况下,对甲虫袭击的反应被证明要大得多(夏季SOA浓度局部增加多达3倍)。放置在来自IMPROVE网络的观察的背景下,与甲虫袭击导致的SOA浓度变化在大多数情况下相比,在北美西部由野火活动驱动的总有机气溶胶存在较大的年度和年度间变化。这表明大多数甲虫引起的SOA变化在当前的观测网络中都不太可能被检测到;但是,这些变化可能会阻碍实现美国西部国家公园和荒野地区自然可见度条件的努力。

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