Vertical profile of tropospheric ozone derived from synergetic retrieval using three different wavelength ranges, UV, IR, and Microwave: sensitivity study for satellite observation

摘要

We performed a quantitative feasibility study of constraining the vertical profile of the amount of ozone in the troposphere by using a synergetic retrieval method on multiple spectra, i.e., ultraviolet (UV), thermal infrared (TIR) and microwave (MW) ranges, measured from space. Twenty atmospheric scenarios for East Asia in summer and winter seasons were assumed in this study. Geometry of line-of-sight was nadir down-looking for UV and TIR measurements, and limb-sounding for MW measurement. The sensitivities of retrieved ozone in the upper troposphere (UT), middle troposphere (MT) and lowermost troposphere (LMT) were estimated using values of the degree of freedom for signal (DFS), partial column error, and averaging kernel matrix, derived based on the optimal estimation method. The measurement noises were assumed at the same level as the currently available instruments. The weighting functions for the UV, TIR and MW ranges were calculated using the SCIATRAN radiative transfer model, the Line-By-Line Radiative Transfer Model, and the Advanced Model for Atmospheric Terahertz Radiation Analysis and Simulation, respectively. In the UT region, the DFS value was enhanced by about 200 % by adding the MW measurements to the combination of UV and TIR measurements. We found that the DFS value of the LMT ozone was increased by approximately 40 % by adding the MW measurements to the combination of UV and TIR measurements; nevertheless, the MW measurement alone has no sensitivity for the LMT ozone. Better information of the LMT ozone can be educed by adding constraints on the UT and MT ozone from the MW measurement. The results of this study will be implemented in the Japanese air-quality monitoring missions, APOLLO, GMAP-Asia and uvSCOPE.