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Simplifying the calculation of light scattering properties for black carbon fractal aggregates

机译:简化黑碳分形聚集体的光散射特性的计算

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摘要

Black carbon fractal aggregates have complicated shapes that make the calculation of their optical properties particularly computationally expensive. Here, a method is presented to estimate fractal aggregate light scattering properties by optimising simplified models to full light scattering calculations. It is found that there are no possible spherical models (at any size or refractive index) that well represent the light scattering in the visible or near-thermal infrared. As such, parameterisations of the light scattering as a function of the number of aggregate particles is presented as the most pragmatic choice for modelling distributions of black carbon when the large computational overheads of rigorous scattering calculations cannot be justified. This parameterisation can be analytically integrated to provide light scattering properties for lognormal distributions of black carbon fractal aggregates and return extinction cross sections with 0.1% accuracy for typical black carbon size distributions. Scattering cross sections and the asymmetry parameter can be obtained to within 3%.
机译:黑碳分形聚集体具有复杂的形状,这使其光学性能的计算特别昂贵。在这里,提出了一种通过优化简化模型以进行全光散射计算来估计分形集合光散射特性的方法。发现没有任何球形模型(任何大小或折射率)都可以很好地表示可见或近红外热中的光散射。因此,当无法证明严格的散射计算的大量计算开销是合理的时,将光散射的参数化设置为聚集颗粒数量的函数,这是对黑碳分布进行建模的最实用的选择。该参数化可以进行分析集成,以为黑碳分形聚集体的对数正态分布和典型的黑碳粒度分布的0.1%精度返回消光截面提供光散射特性。散射截面和不对称参数可以达到3%以内。

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