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Distribution and sources of air pollutants in the North China Plain based onon-road mobile measurements

机译:基于GIS的华北平原大气污染物分布与来源。道路移动测量

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摘要

The North China Plain (NCP) has been experiencing severe airpollution problems with rapid economic growth and urbanisation. Many fieldand model studies have examined the distribution of air pollutants in theNCP, but convincing results have not been achieved, mainly due to a lack ofdirect measurements of pollutants over large areas. Here, we employed amobile laboratory to observe the main air pollutants in a large part of theNCP from 11 June to 15 July 2013. High median concentrations of sulfurdioxide (SO) (12 ppb), nitrogen oxides (NO) (NO + NO;452 ppb), carbon monoxide (CO) (956 ppb), black carbon (BC;5.5 µg m) and ultrafine particles (28 350 cm) weremeasured. Most of the high values, i.e. 95 percentile concentrations, weredistributed near large cities, suggesting the influence of local emissions.In addition, we analysed the regional transport of SO and CO,relatively long-lived pollutants, based on our mobile observations togetherwith wind field and satellite data analyses. Our results suggested that, forborder areas of the NCP, wind from outside this area would have a dilutingeffect on pollutants, while south winds would bring in pollutants that haveaccumulated during transport through other parts of the NCP. For the centralNCP, the concentrations of pollutants were likely to remain at high levels,partly due to the influence of regional transport by prevalent south–northwinds over the NCP and partly by local emissions.
机译:随着经济的快速增长和城市化,华北平原(NCP)一直面临着严重的空气污染问题。许多现场和模型研究已经检查了NCP中空气污染物的分布,但未取得令人信服的结果,这主要是由于缺乏对大面积污染物的直接测量。在这里,我们聘请了一个流动实验室来观察2013年6月11日至7月15日在NCP大部分地区的主要空气污染物。高浓度的二氧化硫(SO)(12 ppb),氮氧化物(NO)(NO + NO; 452) ppb),一氧化碳(CO)(956 ppb),黑碳(BC; 5.5 µg m)和超细颗粒(28 350 cm)进行了测量。大多数高值(即95%浓度)分布在大城市附近,这表明了当地排放的影响。此外,我们根据移动观测和风场分析了SO和CO(相对长寿污染物)的区域迁移和卫星数据分析。我们的结果表明,在NCP的边界区域,来自该区域外部的风将对污染物产生稀释作用,而南风将引入在运输过程中通过NCP其他部分累积的污染物。对于中央NCP,污染物的浓度可能会保持在较高水平,部分原因是受到NCP上普遍的南北风影响的区域运输以及局部排放的影响。

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