Long-term observed ozone trends in the free troposphere and lower stratosphere

摘要

The vertical distributions of ozone trends in the free troposphere and lower stratosphere were derived from ozonesonde observations taken over an average period of approximately 20 years. The results for the annual trends show a consistent pattern of increased ozone of approximately 1 percent/yr to 2 percent/yr up to approximately 300 mb and decreased ozone of approximately -0.6 percent/yr from approximately 100 to 50 mb. Statistically significant positive trends found in midtroposphere (approximately 500 mb) at a set of representative stations in the Northern Hemisphere have little apparent seasonal variation. Negative trends are generally strongest at 50-70 mb with a tendency to be larger during spring. A highly significant negative trend of approximately -5 percent/yr is found near 100 mb over Syowa (69 deg S) during spring.