Full-scale demonstration of the cintichem process for the production of Mo-99 using a low-enriched target

摘要

The irradiation, disassembly, and processing of two full-scale low-enriched uranium (LEU) targets were recently demonstrated by personnel in the BATAN PUSPIPTEK Facilities (Serpong, Indonesia). Targets were fabricated at Argonne National Laboratory (Argonne, IL, U.S.A.) and shipped to PUSPIPTEK. The processing was done by nearly the same procedure used for the production of (sup 99)Mo from high-enriched uranium (HEU) targets. The BATAN Radioisotope Production Centre produces (sup 99)Mo using the Cintichem process by first dissolving the uranium in an acid cocktail; three proprietary separation steps recover the (sup 99)Mo and purify it from other components of the irradiated uranium. Processing of LEU-metal targets is nearly identical to that used for HEU-oxide targets except (1) a separate dissolver is required and (2) the dissolution cocktail is nitric acid alone rather than a nitric /sulfuric acid mixture. The demonstrations went smoothly except for problems with sampling and gamma analysis to assess product purity. Foils could be removed from targets fabricated from zirconium and/or 304 stainless steel, and processing produced an equivalent yield of (sup 99)Mo/(sup 235)U to that of the HEU target.