Design and Construction of an Ultra-Low-Background 14 Germanium Crystal Array for High Efficiency and Coincidence Measurements

摘要

Physics experiments, environmental surveillance, and treaty verification techniques continue to require increased sensitivity for detecting and quantifying radionuclides of interest. This can be done by detecting a greater fraction of gamma emissions from a sample (higher detection efficiency) and reducing instrument backgrounds. A current effort for increased sensitivity in high resolution gamma spectroscopy will produce an intrinsic high-purity germanium (HPGe) array designed for high detection efficiency, ultra-low- background performance, and useful coincidence efficiencies. The system design is optimized to accommodate filter paper samples, e.g., samples collected by the Radionuclide Aerosol Sampler/Analyzer (RASA). The system will provide high sensitivity for weak collections on atmospheric filter samples, as well as offering the potential to gather additional information from more active filters using gamma cascade coincidence detection. The current effort is constructing an ultra-low-background HPGe crystal array consisting of two vacuum cryostats, each housing a hexagonal array of 7 crystals on the order of 70% relative efficiency each. Traditional methods for constructing ultra-low- background detectors are used, including the use of materials known to be low in radioactive contaminants, the use of ultra pure reagents, clean room assembly, etc. The cryostat will be constructed mainly from copper electroformed into near-final geometry at Pacific Northwest National Laboratory (PNN)L. Details of the detector design, simulation of efficiency and coincidence performance, HPGe crystal testing, and progress on cryostat construction are presented.