Monte Carlo study of the magnetic properties of Fe0.9-qMn0.1Alq-disordered alloys

摘要

Within the framework of a random site-diluted Ising model with nearest-neighbor interactions, and using the Metropolis algorithm for equilibration and energy minimization, we have computed the ensemble and configurational averages for magnetization per site, magnetic susceptibility and specific heat of Fe0.9-qMnO0.1Alq-disordered alloys with 0.1 less than or equal to q less than or equal to 0.55. In the model, atoms have been randomly distributed on a body-centered cubic lattice in order to simulate the disorder and structure as that obtained in arc-melted Fe0.9-qMn0.1Alq alloys treated at high temperatures during long periods of time and followed by fast quenching. Competitive interactions coming from Fe-Fe ferromagnetic bonds and Fe-Mn and Mn-Mn antiferromagnetic couplings, as well as the Al dilutor effect, have been taken into account in our study. Results allow us to conclude that, in agreement with previous Mossbauer data of the average hyperfine field, for which a comparison is also carried out, the Fe0.9-qMn0.1Alq-disordered alloys are well characterized by a critical concentration at room temperature at around 40 at% Al, for which the system undergoes a transition from a ferromagnetic state to a paramagnetic one. The finite size scaling analysis to obtain the critical Al concentration in the thermodynamic limit, as well as the critical exponents, is also presented and discussed. (C) 2002 Elsevier Science B.V. All rights reserved. [References: 21]