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Asymmetric spatial distribution in the high-order harmonic generation of a H-2+ molecule controlled by the combination of a mid-infrared laser pulse and a terahertz field

机译:由中红外激光脉冲和太赫兹场组合控制的H-2 +分子高次谐波生成中的不对称空间分布

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摘要

The control of the spatial distribution in the high-order harmonic generation (HHG) of a H-2+ molecule is theoretically investigated by the combination of a mid-infrared laser pulse and a terahertz (THz) field. We use a THz pulse to steer the electron motion, and the numerical results show that the cutoff of the harmonic from the recombination of the electron with the nucleus along the negative-z direction is enhanced and the case along the positive-z direction is suppressed when a THz field is added. The underlying physical mechanism is illustrated by the semi-classical three step model and the ionization probability. The time-frequency analysis further demonstrates the asymmetric spatial distribution in a HHG controlled by adding a THz field.
机译:理论上,通过结合中红外激光脉冲和太赫兹(THz)场,研究了H-2 +分子的高次谐波生成(HHG)中的空间分布控制。我们使用太赫兹(THz)脉冲来控制电子运动,数值结果表明,沿负z方向增强了电子与原子核复合时谐波的截止,并且抑制了沿正z方向的情况添加THz字段时。半经典的三步模型和电离概率说明了潜在的物理机制。时频分析进一步证明了通过添加太赫兹场控制的HHG中的不对称空间分布。

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