In Situ Generation of Ru Nanoparticles to Catalyze CO2 Hydrogenation to Formic Acid

Vivek Srivastava

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In Situ Generation of Ru Nanoparticles to Catalyze CO2 Hydrogenation to Formic Acid

机译：Ru纳米粒子的原位生成催化CO2加氢成甲酸

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Narrow size distributed, stable, catalytically active Ru NPs were synthesis in ionic liquid medium. In situ generated Ru NPs in [DAMI][NTf2] ionic liquid was found highly active in terms of formic acid formed during the CO2 hydrogenation reaction to other ionic liquid immobilized standing Ru NPs. Low catalyst loading, ligand free approach; simple reaction protocol and seven times catalyst recycling are major merits of the proposed work.

机译：在离子液体介质中合成了窄尺寸分布的，稳定的，具有催化活性的Ru NP。发现在[DAMI] [NTf2]离子液体中原位生成的Ru NPs在CO2加氢反应过程中形成的甲酸与固定化其他离子液体的Ru NPs方面具有很高的活性。低催化剂负载，无配体方法;简单的反应方案和七次催化剂循环是拟议工作的主要优点。

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《Catalysis Letters》 |2014年第10期|共6页
作者
Vivek Srivastava;
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正文语种 eng
中图分类催化;
关键词
Ru nanoparticles; Ionic liquid; Formic acid; Carbon sequestration; Carbon dioxide;

机译：钌纳米颗粒;离子液体;甲酸;碳螯合;二氧化碳;

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专利

1. In Situ Generation of Ru Nanoparticles to Catalyze CO2 Hydrogenation to Formic Acid [J] . Vivek Srivastava Catalysis Letters . 2014,第10期

机译：Ru纳米粒子的原位生成催化CO2加氢成甲酸
2. Selective Hydrogenation of CO2 to Formic Acid over Alumina-Supported Ru Nanoparticles with Multifunctional Ionic Liquid [J] . Gautam Prashant, Upadhyay Praveenkumar Ramprakash, Srivastava Vivek Catalysis Letters . 2019,第6期

机译：用多官能离子液体用氧化铝负载的Ru纳米粒子选择性氢化CO2至甲酸
3. Intramolecular N-H...H-Ru proton-hydride interaction in ruthenium complexes with (2-(dimethylamino)ethyl)cyclopentadienyl and (3-(dimethylamino)propyl)cyclopentadienyl ligands. Hydrogenation of CO2 to formic acid via the N-H...H-Ru hydrogen-bonded co [J] . Chu HS., Wong KY., Wong WT., Organometallics . 1998,第13期

机译：钌与（2-（二甲基氨基）乙基）环戊二烯基和（3-（二甲基氨基）丙基）环戊二烯基配体的钌配合物中的分子内N-H ... H-Ru质子-氢化物相互作用。通过N-H ... H-Ru氢键合钴将CO2加氢成甲酸
4. Hydrogenation of Carboxylic Acids Catalyzed by Magnesia-SupportedPoly-γ-Aminopropylsiloxane-Ru Complex [C] . Baowei Mao 11th International Symposium of Fine Chemistry and Functional Polymers Jul 28-31, 2001 Hailar, Inner Mongolia, P.R. China . 2001

机译：氧化镁负载的聚-γ-氨基丙基硅氧烷-钌配合物催化的羧酸加氢反应
5. 1. Reduction of Tertiary Benzamides to Benzaldehydes by an in situ-Generated Schwartz Reagent (Cp2 Zirconium (Hydrogen)Chloride); Formal Synthesis of Lysergic Acid. 2. Ru-Catalyzed Amide-Directed Aryl Carbon-Hydrogen, Carbon-Nitrogen and Carbon-Oxygen Bond Functionalizations: C-B Formation, Carbon-Carbon Suzuki Cross Coupling and Hydrodemethoxylation [D] . Zhao, Yigang 2011

机译：1.通过原位生成的Schwartz试剂（Cp2氯化锆（氢）氯化物）将叔苄酰胺还原为苯甲醛；麦角酸的正式合成。 2. Ru催化的酰胺基芳烃碳氢，碳氮和碳氧键功能化：C-B形成，碳-碳铃木交叉偶联和加氢脱甲氧基化
6. Challengesin the Greener Production of Formates/FormicAcid Methanol and DME by Heterogeneously Catalyzed CO2 Hydrogenation Processes [O] . Andrea Álvarez, Atul Bansode, Atsushi Urakawa, -1

机译：挑战性在格式/格式的绿色生产中非均相催化CO2加氢工艺制得的酸甲醇和DME
7. Enhanced Catalytic Hydrogenation Performance of Rh-Co2O3 Heteroaggregate Nanostructures by in Situ Transformation of Rh@Co CoreShell Nanoparticles [O] . -1

机译：RH-CO CORESHELL纳米粒子原位转化提高RH-CO2O3杂芳氧态纳米结构的催化氢化性能
8. Noble metal catalyzed hydrogen generation from formic acid in nitrite-containing simulated nuclear waste media [R] . King, R. B. , Bhattacharyya, N. K. , Wiemers, K. D. 1994

机译：贵金属催化从含亚硝酸盐的模拟核废料中的甲酸生成氢气

In Situ Generation of Ru Nanoparticles to Catalyze CO2 Hydrogenation to Formic Acid

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