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Reduced graphene oxide modified platinum catalysts for the oxidation of volatile organic compounds

机译:氧化石墨烯改性的还原铂催化剂,用于挥发性有机化合物的氧化

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In this work, we report the synthesis of reduced graphene oxide (rGO) modified platinum (Pt) catalysts for decreasing the temperature of the complete conversion of benzene. The X-ray photoelectron spectroscopy (XPS) analysis reveals the presence of electron transfer between rGO and Pt, which has a significant effect on the catalytic activity. The electron transfer is also proved by Raman spectra in term of the shifting of G-band belonging to the rGO. H-2-temperature programmed reduction (H-2-TPR) results indicate that the rGO facilitates the reduction of surface oxygen over the catalyst. Moreover, increasing the concentration of rGO within a certain range has a positive influence on the catalytic activity. (C) 2015 Elsevier B.V. All rights reserved.
机译:在这项工作中,我们报告了还原型氧化石墨烯(rGO)改性铂(Pt)催化剂的合成,以降低苯的完全转化温度。 X射线光电子能谱(XPS)分析揭示了rGO和Pt之间存在电子转移,这对催化活性具有重要影响。电子传递还通过拉曼光谱证明了属于rGO的G波段的位移。 H-2-程序升温还原(H-2-TPR)结果表明,rGO促进了催化剂表面氧的还原。而且,在一定范围内增加rGO的浓度对催化活性具有积极的影响。 (C)2015 Elsevier B.V.保留所有权利。

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